Dr. Anca ALDEA
Scientific Researcher
Laboratory of Functional Nanostructures
anca[DOT]aldea[AT]infim[DOT]roProjects
1. BIONMEM – Ionophore embedded membranes for ion sensing in biological fluids
Project Type: PD, Start Date: 2022-04-01 End Date: 2024-03-31
Publications
1. Novel cells integrated biosensor based on superoxide dismutase on electrospun fiber scaffolds for the electrochemical screening of cellular stress
Authors:
Sanz, CG; Aldea, A; Oprea, D; Onea, M; Enache, AT; Barsan, MM
Published: JAN 15 2023, BIOSENSORS & BIOELECTRONICS, 220, 114858, DOI: 10.1016/j.bios.2022.114858
A novel electrochemical biosensor was developed to monitor fibroblast cells stress levels for the first time in situ under external stimuli based on the recognition of superoxide anion released upon cell damage. The biosensor comprised metallized polycaprolactone electrospun fibers covered with zinc oxide for improved cell adhesion and signal transduction, whilst stable bioconjugates of mercaptobenzoic acid-functionalized gold nanoparticles/ superoxide dismutase were employed as recognition bioelements. Biosensors were first tested and optimized for in situ generated superoxide detection by fixed potential amperometry at +0.3 V, with minimal interferences from electroactive species in cell culture media. L929 fibroblast cells were then implanted on the optimized biosensor surface and the biosensor morphologically characterized by scanning electron microscopy (SEM) and fluorescence microscopy, which illustrated the network-type pattern of fibroblasts adjacent to the fiber scaffold. Fibroblast stress was induced by zymosan and monitored at the cells integrated biosensor using fixed potential amperometry (CA) with a sensitivity of 26 nA cm-2 mu g mL-1 zymosan and electrochemical impedance spectros-copy (EIS), with similar sensitivity of the biosensor considering the Rs and Z' parameters of around 0.13 omega cm2 mu g-1 mL and high correlation factors R2 of 0.9994. The obtained results underline the applicability of the here developed biosensor for the electrochemical screening of the fibroblast cells stress. The concept in using low-cost biocompatible polymeric fibers as versatile scaffolds for both enzyme immobilization and cell adhesion, opens a new path in developing biosensors for the in-situ investigation of a variety of cellular events.
2. Interface effects on the energy spectrum and quantum transport in two-dimensional topological heterostructures
Authors:
Ostahie, B; Aldea, A
Published: JUN 15 2022, APPLIED SURFACE SCIENCE, 587, 152769, DOI: 10.1016/j.apsusc.2022.152769
We theoretically investigate the spectral and quantum transport properties of two-dimensional heterostructures build up of different topological materials. Surprising behavior arises due to particular tuning of the edge states, provided by internal symmetries or an external magnetic field, in the different constituents of the heterostructure. Specifically, we use the Chern-type topological insulator and the Weyl semimetals with one or two interfaces interposed between these systems. The energy spectrum may contain gaps which exhibit edge states of alternating chirality or, on the contrary, of a given chirality everywhere in the spectrum. Then, the calculation predicts that the quantum Hall effect may lack the negative plateaus or show asymmetric plateaus in the lower and upper part of the spectrum. Also, the channel distribution on the finite size system with interfaces and attached leads may give rise to fractional values of the quantum Hall resistance. The calculations are based on a diatomic lattice model, with hopping to the nearest-and next-nearest-neighbors, exposed to an internal periodic flux (of Haldane-type), and also to an external magnetic field.
3. Disposable superoxide dismutase biosensors based on gold covered polycaprolactone fibers for the detection of superoxide in cell culture media
Authors:
Sanz, CG; Onea, M; Aldea, A; Barsan, MM
Published: MAY 1 2022, TALANTA, 241, 123255, DOI: 10.1016/j.talanta.2022.123255
A novel and disposable biosensor based on superoxide dismutase (SOD) immobilized on gold metallized polycaprolactone electrospun polymeric fibers (PCl/Au) has been developed for the determination of superoxide (O-2(center dot-)) in cell culture media. SOD biosensors were constructed employing three immobilization methods: crosslinking with EDC/NHS at a cysteine self-assembled monolayer (PCl/Au/SODCYS), biopolymer encapsulation with chitosan (PCl/Au/SODCHI) and cross-linking with glutaraldehyde (PCl/Au/SODGA). Scanning electron microscopy was performed at the three different biosensors to evaluate their surface morphologies. Biosensors were employed for the electrochemical detection of superoxide by fixed potential amperometry at different applied potentials, with two distinct enzymatic mechanisms being proposed: i) the reduction of the enzymatically generated peroxide, at -0.3 V, for which the PCl/Au/SODCHI biosensor presented the highest value of sensitivity of 40.1 mu A mM(-1) cm(-2), and ii) the regeneration of the enzyme catalytic copper centre, at +0.3 V, for which the PCl/Au/SODCYS biosensor had the highest sensitivity value of 16.1 mu A mM(-1) cm(-2). The proposed recognition mechanisms were further confirmed by cyclic voltammetric measurements, which enabled also to determine the amount of immobilized electroactive SOD, with highest value corresponding to the PCl/Au/SODCYS biosensor. The biosensors with best analytical performance, PCl/Au/SODCYS and PCl/Au/SODCHI, were further investigated for stability and selectivity, with best results for the PCl/Au/SODCYS, chosen for superoxide monitoring in cell culture media. The study is promising for future application of PCl/Au/SODCYS for the on-line superoxide monitoring of superoxide in cell cultures, grown directly on the biosensor itself.
4. Spectral analysis, chiral disorder and topological edge states manifestation in open non-Hermitian Su-Schrieffer-Heeger chains
Authors:
Ostahie, B; Aldea, A
Published: JAN 28 2021, PHYSICS LETTERS A, 387, DOI: 10.1016/j.physleta.2020.127030
We investigate topological and disorder effects in non-Hermitian systems with chiral symmetry. The system under consideration consists in a finite Su-Schrieffer-Heeger chain to which two semi-infinite leads are attached. The system lacks the parity-time and time-reversal symmetries and is appropriate for the study of quantum transport properties. The complex energy spectrum is analyzed in terms of the chain-lead coupling and chiral disorder strength, and shows substantial differences between chains with even and odd number of sites. The mid-gap edge states acquire a finite lifetime and are both of topological origin or generated by a strong coupling to the leads. The disorder induces coalescence of the topological eigenvalues, associated with exceptional points and vanishing of the eigenfunction rigidity. The electron transmission coefficient is approached in the Landauer formalism, and an analytical expression for the transmission in the range of topological states is obtained. Notably, the chiral disorder in this non-Hermitian system induces unitary conductance enhancement in the topological phase. (C) 2020 Elsevier B.V. All rights reserved.
5. Gold coated electrospun polymeric fibres as new electrode platform for glucose oxidase immobilization
Authors:
Aldea, A; Leote, RJB; Matei, E; Evanghelidis, A; Enculescu, I; Diculescu, VC
Published: JUN 2021, MICROCHEMICAL JOURNAL, 165, 106108, DOI: 10.1016/j.microc.2021.106108
Fibres of poly(methyl methacrylate) were obtained by electrospinning, subjected to coating with a gold layer and then attached on a thin polyethylene terephthalate substrate in order to obtain flexible electrodes for biosensing applications. The morphology of these electrodes, investigated by scanning electron microscopy showed multilayers of random oriented fibres of approx. 400 nm diameter. The electrochemical characterization of these flexible electrodes was performed by cyclic voltammetry and electrochemical impedance spectroscopy in acid and neutral media, in the absence and in the presence of redox probes, proving their superior performance (e.g. 5fold current density value) when compared to planar gold electrodes obtained on silicon wafers. The electrodes obtained from conductive electrospun polymeric fibres nets were tested by cyclic voltammetry and amperometry for the detection of hydrogen peroxide with a sensitivity of 0.84 mA cm-2 mM-1 and a detection limit of 20.40 ?M. The immobilization of the model enzyme glucose oxidase at the surface of the gold-coated electrospun polymeric fibres electrode was investigated and the obtained biosensor was applied for glucose determination in aqueous solutions by fixed potential amperometry with a sensitivity of 3.10 ?A cm-2 mM-1, a detection limit of 0.33 mM, and reduced interferences. Also, the practical applicability of the biosensor was tested for the detection of glucose in artificial sweat and serum samples.
6. Ionophore- Nafion (TM) modified gold-coated electrospun polymeric fibers electrodes for determination of electrolytes
Authors:
Aldea, A; Matei, E; Leote, RJB; Rau, I; Enculescu, I; Diculescu, VC
Published: DEC 10 2020, ELECTROCHIMICA ACTA, 363, 137239, DOI: 10.1016/j.electacta.2020.137239
The present work describes the electrochemical properties of ionophores immobilized at the surface of electrodes obtained from electrospun polymeric fibers, in order to develop sensors for the analysis of electrolytes. Poly(methyl methacrylate) submicrometer fibers were prepared by electrospinning, coated with a gold layer by magnetron sputtering and then transferred on polyethylene terephthalate (PET) in order to obtained flexible electrodes. The ionophores were immobilized at the surface of these electrodes by drop-casting a ionophore-Nafion mixed solution. The sensor surface was investigated by scanning electron microscopy coupled with energy-dispersive X-ray spectroscopy in order to understand the morphology and distribution of a model Ca2+ ionophore over the electrode surface. Also, Fourier-transformed infrared spectroscopy was performed and demonstrated that the model Ca2+ ionophore can be immobilized in the nafion matrix maintaining its conformation, while cyclic voltammetry and electrochemical impedance spectroscopy demonstrated that the Ca2+ ionophore allows the diffusion of target ions through this this type of membrane. In order to prove the concept of ionophore-based sensors for the analysis of some electrolytes, Ca2+, NH4+, Cl- and H+ ionophore immobilized in a nafion matrix at the surface of these flexible electrodes were tested and the determination of the target ions performed by potentiometry in different media including artificial sweat. Finally, sensitivities, limits of detection, selectivity coefficients were determined. (C) 2020 Elsevier Ltd. All rights reserved.
7. Edge-state mechanism for the anomalous quantum Hall effect in a diatomic square lattice
Authors:
Ostahie, B; Nita, M; Aldea, A
Published: SEP 4 2018, PHYSICAL REVIEW B, 98, DOI: 10.1103/PhysRevB.98.125403
We investigate the spectral and transport properties of a diatomic square lattice with hopping to the next-nearest-neighbors and broken time-reversal symmetry, which behaves as a Chern insulator. In a finite-size approach, the attention is paid to the formation of chiral edge states in the topological insulating phase, but also in the semimetallic one. The edge states are revealed in the ribbon and plaquette geometries by analytical and numerical methods, significant differences being produced by the specific atomic connectivity at the boundary. The Hall resistance R-H is calculated in the plaquette geometry using the Landauer-Mittiker approach. The chiral edge states located in the unique gap of the energy spectrum manifest themselves by quantized values R-H = +/- h/e(2) specific to the Chern insulator. The semimetallic system containing chiral edge states embedded in the quasicontinuum of bulk states shows a disorder-driven AQHE as a consequence of the Anderson localization process.
8. Localization Properties of Zig-Zag Edge States in Disordered Phosphorene
Authors:
Nita, M; Ostahie, B; Tolea, M; Aldea, A
Published: JUL 2018, PHYSICA STATUS SOLIDI-RAPID RESEARCH LETTERS, 12, DOI: 10.1002/pssr.201800051
Herein, the spectral and transport properties in the finite phosphorene lattice are investigated using the tight-binding model in the presence of Anderson disorder potential. The focus is on the zig-zag edge states localization, provided by the numerically calculated inverse participation number. At low disorder, the zig-zag states undergo a localization process, keeping their 1D character, while further increasing the disorder leads to delocalization due to hybridization with the extended 2D states. The disorder-induced changes in the electronic conductance, from one zig-zag edge to the other, are also discussed.
9. Phosphorene confined systems in magnetic field, quantum transport, and superradiance in the quasiflat band
Authors:
Ostahie, B; Aldea, A
Published: FEB 2 2016, PHYSICAL REVIEW B, 93, DOI: 10.1103/PhysRevB.93.075408
Spectral and transport properties of electrons in confined phosphorene systems are investigated in a five hopping parameter tight-binding model, using analytical and numerical techniques. The main emphasis is on the properties of the topological edge states accommodated by the quasiflat band that characterizes the phosphorene energy spectrum. We show, in the particular case of phosphorene, how the breaking of the bipartite lattice structure gives rise to the electron-hole asymmetry of the energy spectrum. The properties of the topological edge states in the zigzag nanoribbons are analyzed under different aspects: degeneracy, localization, extension in the Brillouin zone, dispersion of the quasiflat band in magnetic field. The finite-size phosphorene plaquette exhibits a Hofstadter-type spectrum made up of two unequal butterflies separated by a gap, where a quasiflat band composed of zigzag edge states is located. The transport properties are investigated by simulating a four-lead Hall device (importantly, all leads are attached on the same zigzag side), and using the Landauer-Buttiker formalism. We find out that the chiral edge states due to the magnetic field yield quantum Hall plateaus, but the topological edge states in the gap do not support the quantum Hall effect and prove a dissipative behavior. By calculating the complex eigenenergies of the non-Hermitian effective Hamiltonian that describes the open system (plaquette+leads), we prove the superradiance effect in the energy range of the quasiflat band, with consequences for the density of states and electron transmission properties.
10. Non-Hermitian approach of edge states and quantum transport in a magnetic field
Authors:
Ostahie, B; Nita, M; Aldea, A
Published: NOV 21 2016, PHYSICAL REVIEW B, 94, DOI: 10.1103/PhysRevB.94.195431
We develop a manifest non-Hermitian approach of spectral and transport properties of two-dimensional mesoscopic systems in a strong magnetic field. The finite system to which several terminals are attached constitutes an open system that can be described by an effective Hamiltonian. The lifetime of the quantum states expressed by the energy imaginary part depends specifically on the lead-system coupling and makes the difference among three regimes: resonant, integer quantum Hall effect, and superradiant. The discussion is carried on in terms of edge state lifetime in different gaps, channel formation, role of hybridization, and transmission coefficients quantization. A toy model helps in understanding non-Hermitian aspects in open systems.
11. Electrical manipulation of edge states in graphene and the effect on quantum Hall transport
Authors:
Ostahie, B; Nita, M; Aldea, A
Published: APR 9 2015, PHYSICAL REVIEW B, 91, DOI: 10.1103/PhysRevB.91.155409
We investigate the properties of Dirac electrons in a finite graphene sample under a perpendicular magnetic field that emerge when an in-plane electric bias is also applied. The numerical analysis of the Hofstadter spectrum and of the edge-type wave functions evidence the presence of shortcut edge states that appear under the influence of the electric field. The states are characterized by a specific spatial distribution, which follows only partially the perimeter, and exhibit ridges that connect opposite sides of the graphene plaquette. Two kinds of such states have been found in different regions of the spectrum, and their particular spatial localization is shown along with the diamagnetic moments that reveal their chirality. By simulating a four-lead Hall device, we investigate the transport properties and observe unconventional plateaus of the integer quantum Hall effect that are associated with the presence of the shortcut edge states. We show the contributions of the novel states to the conductance matrix that determine the new transport properties. The shortcut edge states resulting from the splitting of the n = 0 Landau level represent a special case, giving rise to nontrivial transverse and longitudinal resistance.
12. Topological properties of the mesoscopic graphene plaquette: Quantum spin Hall effect due to spin imbalance
Authors:
Ostahie, B; Nita, M; Aldea, A
Published: APR 15 2014, PHYSICAL REVIEW B, 89, DOI: 10.1103/PhysRevB.89.165412
We study the electronic properties of the confined honeycomb lattice in the presence of the intrinsic spin-orbit (ISO) interaction and perpendicular magnetic field, and report on uncommon aspects of the quantum spin Hall conductance corroborated by peculiar properties of the edge states. The ISO interaction induces two specific gaps in the Hofstadter spectrum, namely the "weak" topological gap defined by Beugeling et al. [Phys. Rev. B 86, 075118 (2012)], and spin-imbalanced gaps in the relativistic range of the energy spectrum. We analyze the evolution of the helical states with the magnetic field and with increasing Anderson disorder. The "edge" localization of the spin-dependent states and its dependence on the disorder strength is shown. The quantum transport, treated in the Landauer-Buttiker formalism, reveals interesting new plateaus of the quantum spin Hall effect (QSHE), and also of the integer quantum Hall effect (IQHE), in the energy ranges corresponding to the spin-imbalanced gaps. The properties of the spin-dependent transmittance matrix that determine the symmetries with respect to the spin, energy, and magnetic field of the longitudinal and transverse resistance are shown.
13. Spectral and transport properties of the two-dimensional Lieb lattice
Authors:
Nita, M; Ostahie, B; Aldea, A
Published: MAR 29 2013, PHYSICAL REVIEW B, 87, DOI: 10.1103/PhysRevB.87.125428
The specific topology of the line-centered square lattice (known also as the Lieb lattice) induces remarkable spectral properties such as the macroscopically degenerated zero-energy flat band, the Dirac cone in the low-energy spectrum, and the peculiar Hofstadter-type spectrum in a magnetic field. We study here the properties of the finite Lieb lattice with periodic and vanishing boundary conditions. We investigate the behavior of the flat band induced by disorder and external magnetic and electric fields. We show that in the confined Lieb plaquette threaded by a perpendicular magnetic flux there are edge states with nontrivial behavior. The specific class of twisted edge states, which have alternating chirality, are sensitive to disorder and do not support integer quantum Hall effect (IQHE), but contribute to the longitudinal resistance. The symmetry of the transmittance matrix in the energy range where these states are located is revealed. The diamagnetic moments of the bulk and edge states in the Dirac-Landau domain, and also of the flat states in crossed magnetic and electric fields are shown. DOI: 10.1103/PhysRevB.87.125428
14. Phase extraction in disordered isospectral shapes
Authors:
Tolea, M; Ostahie, B; Nita, M; Tolea, F; Aldea, A
Published: MAR 14 2012, PHYSICAL REVIEW E, 85, DOI: 10.1103/PhysRevE.85.036604
The phase of the electronic wave function is not directly measurable but, quite remarkably, it becomes accessible in pairs of isospectral shapes, as recently proposed in the experiment by Moon et al. [Science 319, 782 (2008)]. The method is based on a special property, called transplantation, which relates the eigenfunctions of the isospectral pairs, and allows us to extract the phase distributions, if the amplitude distributions are known. We numerically simulate such a phase extraction procedure in the presence of disorder, which is introduced both as Anderson disorder and as roughness at edges. With disorder, the transplantation can no longer lead to a perfect fit of the wave functions, however we show that a phase can still be extracted-defined as the phase that minimizes the misfit. Interestingly, this extracted phase coincides with (or differs negligibly from) the phase of the disorder-free system, up to a certain disorder amplitude, and a misfit of the wave functions as high as similar to 5%, proving a robustness of the phase extraction method against disorder. However, if the disorder is increased further, the extracted phase shows a puzzle structure, no longer correlated with the phase of the disorder-free system. A discrete model is used, which is the natural approach for disorder analysis. We provide a proof that discretization preserves isospectrality and the transplantation can be adapted to the discrete systems.
15. Fano-Kondo oscillations of the conductance and thermopower in a mesoscopic transistor
Authors:
Aldea, A; Tolea, M; Dinu, IV
Published: 2012, 14TH INTERNATIONAL CONFERENCE ON TRANSPORT IN INTERACTING DISORDERED SYSTEMS (TIDS-14), 376, DOI: 10.1088/1742-6596/376/1/012019
We study the conductance G and Seebeck coefficient S of a side-coupled double quantum dot system. The transport properties are the result of the competition between the Fano interference and Kondo correlations, being also controlled by the Coulomb blockade of the multilevel side-dot. The external parameters are the gate potential V-g applied on the side-dot and the temperature. When V-g is varied continuously the blockade is switched on and off periodically, resulting in oscillations of the transport coefficients. The profile of the oscillations and the temperature dependence are studied. An extended Anderson model and the Keldysh transport formalism are used.
16. Zero bias anomalies in the Kondo regime of single and double quantum dots
Authors:
Aldea, A; Tolea, M; Dinu, IV
Published: 2012, ADVANCED MANY-BODY AND STATISTICAL METHODS IN MESOSCOPIC SYSTEMS, 338, DOI: 10.1088/1742-6596/338/1/012001
The zero bias anomaly of the differential conductance of mesoscopic systems is a fingerprint of the electron-electron interaction. The common example is the peak of the differential conductance in Kondo mesoscopic systems. We show that in complex mesoscopic systems, in particular in the side-coupled double dot, the dip of the differential conductance at zero bias is also possible due to simultaneous effects of interference and correlations. The external parameters that control this effect are the temperature and the gate potential on the lateral dot. We argue that even in single dots, in a multiple lead configuration, the shift from suppression to enhancement of dI/dV with increasing bias is allowed if the bias applied on the leads is not symmetric. The differential conductance exhibits a peak-dip crossover, the effect being controlled by the strength of the asymmetry and the ratio of the dot-lead couplings. The scaling of the differential conductance for the double-dot system is also discussed. The results are obtained using an extended Anderson model, the Keldysh transport formalism and the equation of motion technique extended to the non-equilibrium.
17. Coulomb oscillations in the Fano-Kondo effect and zero-bias anomalies in a double-dot mesotransistor
Authors:
Aldea, A; Tolea, M; Dinu, IV
Published: JUN 27 2011, PHYSICAL REVIEW B, 83, DOI: 10.1103/PhysRevB.83.245317
We investigate theoretically the transport properties of the side-coupled double quantum dots in connection with the experimental study of Sasaki et al. [Phys. Rev. Lett. 103, 266806 (2009)]. The setup consists of connecting the Kondo dot directly to the leads, while the side dot provides an interference path which affects the Kondo correlations. We analyze the oscillations of the source-drain current due to the periodical Coulomb blockade of the many-level side dot at the variation of the gate potential applied on it. The Fano profile of these oscillations may be controlled by the interdot coupling, level spacing of the side dot, and also by the temperature. The nonequilibrium conductance of the double-dot system exhibits zero-bias anomaly which, besides the usual enhancement, may show also a suppression (a diplike aspect) which occurs around the Fano zero. In the same region, the weak temperature dependence of the conductance indicates the suppression of the Kondo effect. Scaling properties of the nonequilibrium conductance in the Fano-Kondo regime are discussed. Since the Kondo temperature of the single-impurity Anderson model is no longer the proper scaling parameter, we look for an alternative specific to the double dot. The extended Anderson model, Keldysh formalism, and equation-of-motion technique are used.
18. Analyzing the measured phase in the multichannel Aharonov-Bohm interferometer
Authors:
Tolea, M; Nita, M; Aldea, A
Published: JUL 2010, PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 42, 2236, DOI: 10.1016/j.physe.2010.04.022
We address the quantum dot phase measurement problem in an open Aharonov-Bohm interferometer, assuming multiple transport channels. In such a case, the quantum dot is characterized by more than one intrinsic phase for the electrons transmission. It is shown that the phase which would be extracted by the usual experimental method (i.e. by monitoring the shift of the Aharonov-Bohm oscillations, as in Schuster et al., Nature 385 (1997) 417) does not coincide with any of the dot intrinsic phases, but is a combination of them. The formula of the measured phase is given. The particular case of a quantum dot containing a S = 1/2 spin is discussed and variations of the measured phase with <pi are found, as a consequence of the multichannel transport. (C) 2010 Elsevier B.V. All rights reserved.
19. Kondo peaks and dips in the differential conductance of a multi-lead quantum dot: Dependence on bias conditions
Authors:
Tolea, M; Dinu, IV; Aldea, A
Published: JAN 2009, PHYSICAL REVIEW B, 79, DOI: 10.1103/PhysRevB.79.033306
We study the differential conductance in the Kondo regime of a quantum dot coupled to multiple leads. When the bias is applied symmetrically on two of the leads (V and -V, as usual in experiments) while the others are grounded, the conductance through the biased leads always shows the expected enhancement at zero bias. However, under asymmetrically applied bias (V and lambda V, with lambda>0), a suppression-dip-appears in the differential conductance if the asymmetry coefficient lambda is beyond a given threshold lambda(0)=3 root 1+r determined by the ratio r of the dot-lead couplings. This is a recipe to determine experimentally this ratio which is important for the quantum-dot devices. This finding is a direct result of the Keldysh transport formalism. For the illustration we use a many-lead Anderson Hamiltonian, the Green's functions being calculated in the Lacroix approximation, which is generalized to the case of nonequilibrium.
20. Peak-dip crossover of the differential conductance in mesoscopic systems with quantum impurities
Authors:
Aldea, A; Tolea, M; Dinu, IV
Published: 2009, 25TH INTERNATIONAL CONFERENCE ON LOW TEMPERATURE PHYSICS (LT25), PART 2, 150, DOI: 10.1088/1742-6596/150/2/022001
We investigate the differential conductance dI/dV for the interacting T-shape model, using an approach based on the Keldysh formalism and the Lacroix solution for the equation of motion. A peak-dip crossover has been noticed by changing the hybridization between the two dots. For the same model, the combined interaction and interference processes give rise to the Fano-Kondo effect with an interesting crossing point of the isoterms below the Kondo temperature A tentative explanation of these effects is given in terms of the many-body spectral properties of the system.
21. Transport through quantum dots with magnetic impurities
Authors:
Tolea, M; Aldea, A; Bulka, BR
Published: JUL 2008, JOURNAL OF OPTOELECTRONICS AND ADVANCED MATERIALS, 10, 1758, DOI:
We analyze the electronic transport through a quantum dot that contains a magnetic impurity. The coherent transport of electrons is governed by the quantum confinement inside the dot, but is also influenced by the exchange interaction with the impurity. The interplay between the two gives raise to the singlet-triplet splitting of the energy levels available for the tunneling electron. In this paper, we focus on the charge fluctuations and, more precisely, the height of the conductance peaks. We show that the conductance peaks corresponding to the triplet levels are three times higher than those corresponding to singlet levels, if electronic correlations are neglected (for non-interacting dots, when an exact solution can be obtained). Next, we consider the Coulomb repulsion and the many-body correlations. In this case, the singlet/triplet peak height ratio has a complex behavior. Usually the highest peak corresponds to the state that is lowest in energy (ground state), regardless if it is singlet or triplet. In the end, we get an insight on the Kondo regime for such a system, and show the formation of three Kondo peaks. We use the equation of motion method with appropriate decoupling.
22. Transport through a multiply connected interacting mesoscopic system using the Keldysh formalism
Authors:
Dinu, IV; Tolea, M; Aldea, A
Published: SEP 2007, PHYSICAL REVIEW B, 76, DOI: 10.1103/PhysRevB.76.113302
We apply the Keldysh formalism in order to derive a current formula easy to use for a system with many sites, one of which is interacting. The main technical challenge is to deal with the lesser Green's function. It turns out that, in the case of the left-right symmetry, the knowledge of the lesser Green's function is not necessary and an exact current formula can be expressed in terms of retarded Green's functions only. The application is done for a triangular interferometer which gives a good account of the Fano-Kondo effect. It is found that the interference effects, in the context of Kondo correlations, give rise to a point in the parameter space where the conductance is temperature independent. We include a comparison with the results from Ng's ansatz [Phys. Rev. Lett. 70, 3635 (1993)], which are less accurate, but can be used also in the absence of the above mentioned symmetry.
23. Asymmetric localization in disordered Landau bands
Authors:
Nita, M; Aldea, A; Zittartz, J
Published: JUN 6 2007, JOURNAL OF PHYSICS-CONDENSED MATTER, 19, DOI: 10.1088/0953-8984/19/22/226217
We show that, due to band mixing, the eigenstate localization within the disordered Landau bands gets an asymmetric structure: the degree of localization increases in the lower part of the band and decreases in the upper one. The calculation is performed for a two-dimensional lattice with the Anderson disorder potential and we prove that this effect is related to the upper shift of the extended states within the band and is enhanced by the disorder strength. The asymmetric localization and the energy shift disappear when the interband coupling is switched off.
24. Mesoscopic Fano effect in Aharonov-Bohm rings with an embedded double dot
Authors:
Tanatar, B; Moldoveanu, V; Tolea, M; Aldea, A
Published: 2006, LOW TEMPERATURE PHYSICS, PTS A AND B, 850, +, DOI:
We investigate theoretically in a tight-binding model the transport properties of the Aharonov-Bohm interferometer (ABI) with one dot embedded in each of its arms. For weak interdot coupling the model Hamiltonian describes the system considered in the experiments of Holleitner et al. [Phys. Rev. Lett. 87, 256802 (2001)]. The electronic transmittance of the interferometer is computed within the Landauer-Buttiker formalism while the coexistence of resonant and coherent transport is explicitly emphasized by using the Feschbach formula. The latter produces effective Hamiltonians whose spectral properties describe the tunneling processes through each dot. We reproduce numerically the stability charging diagrams reported in the experiments of Holleitner et al. When the magnetic flux is fixed and one dot is set to resonance the interferometer transmittance shows Fano, lineshapes as a function of the gate voltage applied to the other dot. Our model includes the effect of the magnetic field on the dot levels and explains the change of the asymmetric tail as the magnetic flux is varied. The transmittance assigned to the Fano, dips located in the almost crossing point of the charging diagrams shows Aharonov-Bohm oscillations.
25. Fano interference in mesoscopic rings with quantum dots
Authors:
Moldoveanu, V; Aldea, A; Tolea, M
Published: 2006, PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 3, NO 2, 3, +, DOI: 10.1002/pssc.200562736
We propose a general formalism for describing the coexistence of coherent and resonant transport in hybrid mesoscopic structures. The approach is based on Landauer- Buttiker formula for the electronic transmittance and on an old formula of Feshbach. The latter gives the complete Green function of coupled subsystems in terms of effective Green functions of the disconnected parts and provides informations about the individual contributions of each subsystem to transport. Motivated by the experiments of Kobayashi et al.(Phys. Rev. Lett. 88, 256806 (2002)) and Holleitner et al. (Phys. Rev. Lett. 87, 256802 (2001)) we apply the formalism to study transport in Aharonov-Bohm interferometers (ABI) containing one or two coupled two-dimensional quantum dots (QD). In the single dot case, we reproduce and explain the magnetic field control of the Fano interference and investigate the interaction effects in a self-consistent approach. In the double dot case, we obtain the charging diagrams and establish precise criteria for the observation of mesoscopic Fano effect and AB oscillations. (c) 2006 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
26. Criteria for the occurrence of negative resonant magnetoresistance in magnetic tunnel junctions
Authors:
Tolea, M; Aldea, A; Tolea, F
Published: SEP 2006, PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 243, R86, DOI: 10.1002/pssb.200642347
The dependence of the driven-current through a tunnel junction on the relative orientation of the magnetization in the electrodes deviates from the Julliere formula when the current is resonant through impurity levels. For asymmetric coupling of the impurities to the electrodes, the magnetoresistance can even be negative on the resonance. Such inversion in sign is due to the fact that not only the density of states in the electrodes is important (for both orientations of spins), but also the density of states at the impurity position, which has a specific behavior. We find the exact conditions under which the negative magnetoresistance occurs, as function of both polarization and coupling asymmetry. The resonant magnetoresistance may have single or double-dip aspect, depending on the mentioned parameters.
27. Resonant and coherent transport through Aharonov-Bohm interferometers with coupled quantum dots
Authors:
Moldoveanu, V; Tolea, M; Aldea, A; Tanatar, B
Published: MAR 2005, PHYSICAL REVIEW B, 71, DOI: 10.1103/PhysRevB.71.125338
A detailed description of the tunneling processes, within Aharonov-Bohm (AB) rings containing two-dimensional quantum dots is presented. We show that the electronic propagation through the interferometer is controlled by the spectral properties of the embedded dots and by their coupling with the ring. The transmittance of the interferometer is computed by the Landauer-Buttiker formula. Numerical results are presented for an AB interferometer containing two coupled dots. The charging diagrams for a double-dot interferometer and the Aharonov-Bohm oscillations are obtained, in agreement with the recent experimental results of Holleitner et al. [Phys. Rev. Lett. 87, 256802 (2001)] We identify conditions in which the system shows Fano line shapes. The direction of the asymetric tail depends on the capacitive coupling and on the magnetic field. We discuss our results in connection with the experiments of Kobayashi et al. [Phys. Rev. Lett. 88, 256806 (2002)] in the case of a single dot.
28. Spin magnetoconductance in the mesoscopic spin-interferometer
Authors:
Aldea, A; Tolea, M; Zittartz, J
Published: JUL 2005, PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 28, 202, DOI: 10.1016/j.physe.2005.03.013
We investigate the properties of the electron spin-transmission through an Aharonov-Bohm interferometer with an embedded two-dimensional (2D) multilevel quantum dot containing magnetic impurities. A suitable formalism is developed. The amplitude and the phase of the flip- and non-flip-transmittances are calculated numerically as function of the magnetic field. The effects induced by the exchange interaction and those arising from the 2D character of the dot are shown. (c) 2005 Elsevier B.V. All rights reserved.
29. Disorder effects on the properties of two-dimensional finite systems in perpendicular magnetic field: the tight binding approach
Authors:
Aldea, A; Nita, M; Dinu, V; Tolea, M
Published: JUL 2004, PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 241, 2096, DOI: 10.1002/pssb.200404781
We review some aspects concerning the disorder effects on the spectral properties of 2D electronic systems with relevance for the transport and orbital magnetism in perpendicular magnetic field. The lattice model and random Anderson disorder are used. The discussion is carried out separately for periodic and hard wall boundary conditions. The degree of localization is evidenced by the calculation of the inverse participation number of the eigenstates of the Hamiltonian and a striking asymmetry of the localization effect of states in the Landau band is reported. (C) 2004 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
30. Tunneling properties of quantum dot arrays in a strong magnetic field
Authors:
Moldoveanu, V; Aldea, A; Tanatar, B
Published: AUG 2004, PHYSICAL REVIEW B, 70, DOI: 10.1103/PhysRevB.70.085303
We study the transport properties of coherently coupled quantum dots in the quantum Hall regime within the Landauer-Buttiker formalism which captures and explains the experimentally observed features in terms of the spectral properties of the coupled dot system. The subpeak structure of the transmittance spectrum and the charging stability diagrams are obtained and discussed. The role of the intradot and interdot Coulomb interaction are pointed out. We show the subpeak evolution with the magnetic field and predict a specific oscillatory behavior of the Hall resistance in strong magnetic field which can be experimentally tested.
31. Spin magnetization of a strongly correlated electron gas confined in a two-dimensional finite lattice
Authors:
Nita, M; Dinu, V; Aldea, A; Tanatar, B
Published: FEB 2004, PHYSICAL REVIEW B, 69, DOI: 10.1103/PhysRevB.69.073106
The influence of disorder and interaction effects on the ground state polarization of the two-dimensional correlated electron gas is studied by numerical investigations of the unrestricted Hartree-Fock approach. With the model of Anderson disorder a continuous increase of the spin magnetization until the fully polarized regime is obtained. The ferromagnetic ground state is found to be favorable when the electron number is lowered and the interaction and disorder parameters are suitably chosen.
32. Orbital magnetization of single and double quantum dots in a tight-binding model
Authors:
Aldea, A; Moldoveanu, V; Nita, M; Manolescu, A; Gudmundsson, V; Tanatar, B
Published: JAN 15 2003, PHYSICAL REVIEW B, 67, DOI: 10.1103/PhysRevB.67.035324
We calculate the orbital magnetization of single and double quantum dots coupled both by Coulomb interaction and by electron tunneling. The electronic states of the quantum dots are calculated in a tight-binding model, and the magnetization is discussed in relation to the energy spectrum and to the edge and bulk states. We identify effects of chirality of the electronic orbits and of the anticrossing of the energy levels when the magnetic field is varied. We also consider the effects of detuning the energy spectra of the quantum dots by an external gate potential. We compare our results with the recent experiments of Oosterkamp [Phys. Rev. Lett. 80, 4951 (1998)].
33. Electronic transport in nanosystems
Authors:
Wulf, U; Racec, ER; Racec, PN; Aldea, A
Published: DEC 15 2003, MATERIALS SCIENCE & ENGINEERING C-BIOMIMETIC AND SUPRAMOLECULAR SYSTEMS, 23, 681, DOI: 10.1016/j.msec.2003.09.080
We demonstrate the application of the Landauer-Buttiker formalism (LBF) to MIS (metal-insulator-semiconductor)-type quantum nanostructures and analyze their static and dynamical response properties. For the time-dependent problem, we employ the random phase approximation (RPA) and calculate the irreducible polarization from the one-particle scattering wave functions in the Hartree approximation. For their calculation, we employ the R-matrix approach which we have developed over the past years. We find in the low frequency limit a reasonable agreement with the static Hartree calculations and experimental capacitance data. (C) 2003 Published by Elsevier B.V.
34. Coulomb effects on the transport properties of quantum dots in a strong magnetic field
Authors:
Moldoveanu, V; Aldea, A; Manolescu, A; Nita, M
Published: JAN 15 2001, PHYSICAL REVIEW B, 63, DOI: 10.1103/PhysRevB.63.045301
We investigate the transport properties of quantum dots placed in a strong magnetic field using a quantum-mechanical approach based on the two-dimensional tight-binding Hamiltonian with direct Coulomb interaction and the Landauer-Buttiker formalism. The electronic transmittance and the Hall resistance show Coulomb oscillations and also prove multiple addition processes. We identify this feature as the "bunching" of electrons observed in recent experiments and give an elementary explanation in terms of spectral characteristics of the dot. The spatial distribution of the added electrons may distinguish between the edge and bulk states and it has specific features for bunched electrons. The dependence of the charging energy on the number of electrons is discussed for a strong magnetic field. The crossover from the tunneling to quantum Hall regime is analyzed in terms of dot-lead coupling.
35. Magnetization and level statistics at the quantum Hall liquid-insulator transition in the lattice model
Authors:
Nita, M; Aldea, A; Zittartz, J
Published: DEC 15 2000, PHYSICAL REVIEW B, 62, 15370, DOI: 10.1103/PhysRevB.62.15367
Statistics of level spacing and magnetization are studied for the phase diagram of the integer quantum Hall effect in a two-dimensional finite lattice model with Anderson disorder.
36. Electronic structure of (001) AlAs-InAs-GaAs multilayer structures
Authors:
Velasco, VR; Fernandez-Alvarez, L; Aldea, A; Vlaev, S; Monsivais, G; Garcia-Moliner, F
Published: SEP 3 1998, SURFACE SCIENCE, 412-13, 404, DOI: 10.1016/S0039-6028(98)00458-0
The electronic structure of different (001) (AlAs)(m)(InAs)(1)(GaAs)(m) multilayer structures is studied. We have thus seen the influence of the relative thicknesses of the constituent materials and of the positions of the InAs principal layers in the multilayer structures on the energy eigenstates and on their spatial localization. The calculations are based on an sp(3)s* empirical tight-binding model and on the surface Green function matching method. (C) 1998 Elsevier Science B.V. All rights reserved.
37. QHE, magnetoresistance and disordered transport on 2D mesoscopic plaquettes
Authors:
Aldea, A; Gartner, P; Nita, M
Published: JAN 1998, PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 205, 356, DOI: 10.1002/(SICI)1521-3951(199801)205:1<351::AID-PSSB351>3.3.CO;2-Z
The transport properties of a rectangular mesoscopic plaquette in the presence of a perpendicular magnetic field are studied in a tight-binding model with randomly distributed traps. The longitudinal and Hall resistances are calculated in the four-probe Landauer-Buttiker formalism which accounts automatically both for the quantum coherence and the trapping-induced localization. The localized character of eigenvectors and the specific aspect of the density of states at a given magnetic flux are correlated with the behaviour of the mentioned resistances as function of the Fermi energy. The Hall insulator and quantum Hall regimes are evidenced. The magnetic field dependence of the configurational averages of the longitudinal and Hal; resistance is studied in a purely quantum-mechanical approach. Both, negative and positive magnetoresistances are found.
38. Specific plateaus of the quantum Hall effect induced by an applied bias
Authors:
Aldea, A; Gartner, P; Manolescu, A; Nita, M
Published: MAY 15 1997, PHYSICAL REVIEW B, 55, 13392, DOI: 10.1103/PhysRevB.55.R13389
The spectrum and the eigenstates of a finite two-dimensional tight-binding electronic system, with Dirichlet boundary conditions, in a magnetic field and with an external linear potential are studied. The eigenstates show an equipotential character, and may cross the plaquette in the direction perpendicular to the electric field. When leads are added to the plaquette, the channels carrying the current may be shortcut by equipotentials, resulting in additional plateaus situated between the usual integer-quantum-Hall-effect plateaus. This ideals confirmed by a numerical calculation within the four-terminal Landauer-Buttiker approach.
39. Hall effect and magnetoresistance in four-probe tight-binding mesoscopic rings
Authors:
Gartner, P; Aldea, A
Published: MAR 1996, ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 99, 373, DOI: 10.1007/s002570050050
The Hall effect and magnetoresistance of a mesoscopic system having a four-probe ring geometry are calculated in a tight-binding model, either ordered or disordered, as function of magnetic flux and Fermi energy. The changes induced in the spectrum by the magnetic field affect differently the Aharonov-Bohm (AB) oscillating pattern of the two resistances: after the gap reaches the Fermi energy, the Hall effect remains bounded while the magnetoresistance increases exponentially with the sample size. The results are shown to depend significantly on the number and geometry of the probes.
40. HOPPING CONDUCTIVITY OF THE FIBONACCI-CHAIN QUASI-CRYSTAL - COMMENT
Authors:
DULEA, M; ALDEA, A
Published: OCT 1 1992, PHYSICAL REVIEW B, 46, 8643, DOI: 10.1103/PhysRevB.46.8642
This Comment refers to a recent publication on the ac hopping conduction of the Fibonacci chain [Phys. Rev. B 43, 1183 (1991)]. The renormalization procedure proposed by its authors gives a correct formula for the conductivity [Eq. (15)]. Nevertheless, their conclusion regarding the vanishing of the dc conductivity disagrees with the low-frequency asymptotics previously derived by us for the same model, and also disagrees with the general result given by the resistance-network analogy of the Miller-Abrahams rate equations. Their result assumes the factorization of the frequency in Eq. (15), which we prove is not true. We show also that their numerical curves, which apparently support their conclusion, are strongly influenced by errors in the low-frequency range.
41. THE EFFECT OF THE TEMPERATURE SHIFT OF THE ENERGY-BANDS ON THE THERMOPOWER OF QUASI-FREE ELECTRONS IN SEMICONDUCTORS
Authors:
ALDEA, A
Published: SEP 1989, PHILOSOPHICAL MAGAZINE B-PHYSICS OF CONDENSED MATTER STATISTICAL MECHANICS ELECTRONIC OPTICAL AND MAGNETIC PROPERTIES, 60, 398, DOI: 10.1080/13642818908205915
42. THE THERMOPOWER OF NON-LOCALIZED ELECTRONS IN AMORPHOUS-SEMICONDUCTORS
Authors:
ALDEA, A
Published: DEC 1989, JOURNAL OF NON-CRYSTALLINE SOLIDS, 114, 377, DOI: 10.1016/0022-3093(89)90168-3
43. LONG-TIME ASYMPTOTICS IN THE ONE-DIMENSIONAL TRAPPING PROBLEM WITH LARGE BIAS
Authors:
ALDEA, A; DULEA, M; GARTNER, P
Published: AUG 1988, JOURNAL OF STATISTICAL PHYSICS, 52, 1068, DOI: 10.1007/BF01019739
44. HOPPING CONDUCTION ON APERIODIC CHAINS
Authors:
ALDEA, A; DULEA, M
Published: APR 18 1988, PHYSICAL REVIEW LETTERS, 60, 1675, DOI: 10.1103/PhysRevLett.60.1672
45. PHOTOLUMINESCENCE OF THE HOPPING DISORDERED-SYSTEMS WITH ELECTRICAL BIAS
Authors:
DULEA, M; ALDEA, A
Published: FEB 1987, JOURNAL OF NON-CRYSTALLINE SOLIDS, 90, 464, DOI: 10.1016/S0022-3093(87)80464-7
46. AC CONDUCTIVITY OF A DISORDERED CHAIN - REAL-SPACE RENORMALIZATION-GROUP APPROACH
Authors:
ALDEA, A; DULEA, M
Published: JUL 30 1986, JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 19, 4062, DOI: 10.1088/0022-3719/19/21/010
47. ON THE NYQUIST NOISE
Authors:
BANYAI, L; ALDEA, A; GARTNER, P
Published: 1985, ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 58, 164, DOI: 10.1007/BF01304270
48. ELECTROMAGNETIC EFFECTS IN MAGNETIC SUPERCONDUCTORS
Authors:
ALDEA, A; TURCU, I
Published: 1984, PHYSICAL REVIEW B, 29, 6217, DOI: 10.1103/PhysRevB.29.6213
49. SELF-CONSISTENT MICROSCOPIC APPROACH OF THE MEISSNER EFFECT IN MAGNETIC SUPERCONDUCTORS
Authors:
TURCU, I; ALDEA, A
Published: 1984, PHYSICA A, 126, 528, DOI: 10.1016/0378-4371(84)90216-4
51. A THEORY OF THE RED SHIFT EFFECT IN FERROMAGNETIC SEMICONDUCTORS
Authors:
ALDEA, A; TELEMAN, E
Published: 1980, JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 15-8, 884, DOI: 10.1016/0304-8853(80)90807-0
52. INFLUENCE OF THE S-F INTERACTION ON THE CONDUCTION-BAND BEHAVIOR IN FERROMAGNETIC SEMICONDUCTORS - THEORY OF THE RED SHIFT EFFECT
Authors:
ALDEA, A; TELEMAN, E
Published: 1980, ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 37, 141, DOI: 10.1007/BF01365369
54. MASTER EQUATION APPROACH TO THE HOPPING TRANSPORT-THEORY
Authors:
BANYAI, L; ALDEA, A
Published: 1979, FORTSCHRITTE DER PHYSIK-PROGRESS OF PHYSICS, 27, 462, DOI: 10.1002/prop.19790270903
55. SEMICLASSICAL AND QUANTUM-MECHANICAL THEORY OF HOPPING CONDUCTION
Authors:
BANYAI, L; ALDEA, A
Published: 1977, PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 79, 377, DOI: 10.1002/pssb.2220790139
57. IMPORTANCE OF COULOMB EFFECTS IN TRANSPORT PHENOMENA ON LOCALIZED STATES
Authors:
ALDEA, A; BANYAI, L; CAPEK, V
Published: 1976, CZECHOSLOVAK JOURNAL OF PHYSICS, 26, 720, DOI: 10.1007/BF01589602
58. CONDUCTION-BAND BEHAVIOR IN ANTIFERROMAGNETIC SEMICONDUCTORS
Authors:
TELEMAN, E; ALDEA, A
Published: 1975, JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 8, 52, DOI: 10.1088/0022-3719/8/1/009
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