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Dr. Valeriu MOLDOVEANU

Scientific Researcher I

Studies: Graduate studies, Faculty of Physics, University of Bucharest 1993-1998

               Master Degree in Condensed Matter Physics, University of Bucharest, 1998-2000.

 

Academic degree: PhD in Theoretical Physics: May 24 2004, Universite de la Mediteranee Aix-Marseille II & University of Bucharest, Cotutelle de these, supervised by Prof. Gheorghe Nenciu (University of Bucharest) and Prof. Francois Bentosela (Centre de Physique Theorique - CPT).

Postdoc positions - Technion Institute, Haifa, Israel (May-June 2006)

- Institut for Matematiske Fag, Aalborg, Denmark (September 2010-April 2011).

Current position: Scientific Researcher 1st degree, Head of the Theoretical Physics and Computational Modeling Group, National Institute of Materials Physics.

Research stages abroad:

- NATO - TUBITAK fellowship at Bilkent University (Ankara, Turkey), July-September 2001-2003, 2005.

- NATO Fellowship at Science Institute, Reykjavik, Iceland, November 2004.

- Guest Scientist at Bilkent University, Ankara, Turkey (3 months/year 2007-2009).

- Research Fellow at Science Institute, Reykjavik, Iceland (3-4 moths/year 2006-2010).

Teaching experience: - 2000-2002: Tutoring in „Thermodynamics and Statistical Mechanics'' for

students in their 3rd year at Faculty of Physics, Bucharest.

- 2004: ATER (Attache Temporaire Enseignement et Recherche ) at Universite de Toulon et du Var, France (courses: Series, Statistics and Probabilities ).

 - 2013: Master Courses at the Theoretical Physics Department of the Physics Faculty (University of Bucharest): Non-equilibrium transport in mesoscopic systems, Master equation approach to open systems.

 

 

Radu Grigorovici Prize of the Romanian Academy 2010, (https://acad.ro/premiileAR/liste/2010.pdf)

Quantum transport in nano-devices, Hybrid quantum systems (nano-electromechanical systems, cavity-embedded quantum dots, color centers).

1

Spin configuration of an array of quantum rings controlled by cavity photons

Gudmundsson, V; Mughnetsyan, V; Goan, HS; Chai, JD; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

MAR 11 2025, PHYSICAL REVIEW B, 111, 115304

DOI: 10.1103/PhysRevB.111.115304

Show abstract

We model a change of the spin configuration in a two-dimensional square array, or a lateral superlattice, of quantum rings in an external perpendicular homogeneous magnetic field. The electron system is placed in a circular cylindrical far-infrared photon cavity with a single circularly symmetric photon mode. Our numerical results reveal that the spin ordering of the two-dimensional electron gas in each quantum ring can be influenced or controlled by the electron-photon coupling strength and the energy of the photons. The Coulomb interaction between the electrons is described by a spin-density functional approach, but the para- and diamagnetic electron-photon interactions are modeled via a configuration interaction formalism in a truncated many-body Fock-space, which is updated in each iteration step of the density functional approach. In the absence of external electromagnetic pulses this reordering of the spin configuration is replicated in the orbital magnetization of the rings. The change in the spin configuration can be suppressed by a strong electron-photon interaction. In addition, fluctuations in the spin configuration are found in dynamical calculations, where the system is excited by a time-dependent coupling scheme to a cylindrical cavity mode for emphasizing the diamagnetic electron-photon interaction not leading to simple electrical dipole oscillations. The diamagnetic interaction is enhanced by the rotational electric field of the particular cavity mode.

2 Open Access

Magnetic Properties of A Cavity-Embedded Square Lattice of Quantum Dots or Antidots

Mughnetsyan, V; Gudmundsson, V; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

APR 2024, ANNALEN DER PHYSIK, 536

DOI: 10.1002/andp.202300274

Show abstract

Quantum electrodynamical density functional theory is applied to obtain the electronic density, spin polarization, as well as orbital and spin magnetizations of square periodic arrays of quantum dots or antidots subjected to the influence of a far-infrared cavity photon field. A gradient-based exchange-correlation functional adapted to a 2D electron gas in a transverse homogeneous magnetic field is used in the theoretical framework and calculations. The obtained results predict a non-trivial effect of the cavity field on the electron distribution in the unit cell of the superlattice, as well as on the orbital and spin magnetizations. The number of electrons per unit cell of the superlattice is shown to play a crucial role in the modification of the magnetization via the electron-photon coupling. The calculations show that cavity photons strengthen the diamagnetic effect in the quantum dot structure, while they weaken the paramagnetic effect in the antidot structure. As the number of electrons per unit cell of the lattice increases, the electron-photon interaction reduces the exchange forces that will otherwise promote strong spin splitting for both the dot and the antidot arrays. Electronic density, spin polarization, as well as orbital and spin magnetizations of square periodic arrays of quantum dots or antidots subjected to the influence of a far-infrared cavity photon field are obtained using quantum electrodynamical density functional theory adapted to a 2D electron gas in a transverse homogeneous magnetic field. image

3 Open Access

Magneto-optical properties of a quantum dot array interacting with a far-infrared photon mode of a cylindrical cavity

Gudmundsson, V; Mughnetsyan, V; Goan, HS; Chai, JD; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

JUN 26 2024, PHYSICAL REVIEW B, 109, 235306

DOI: 10.1103/PhysRevB.109.235306

Show abstract

We model the equilibrium properties of a two-dimensional electron gas in a square lateral superlattice of quantum dots in a GaAs heterostructure subject to an external homogeneous perpendicular magnetic field and a far-infrared circular cylindrical photon cavity with one quantized mode, the TE011 mode. In a truncated linear basis constructed by a tensor product of the single-electron states of the noninteracting system and the eigenstates of the photon number operator, a local spin density approximation of density functional theory is used to compute the electron-photon states of the two-dimensional electron gas in the cavity. The common spatial symmetry of the vector fields for the external magnetic field and the cavity photon field in the long wavelength approximation enhances higher order magnetic single- and multiphoton processes for both the para- and the diamagnetic electron-photon interactions. The electron-photon coupling introduces explicit photon replicas into the band structure and all subbands gain a photon content, constant for each subband, that can deviate from an integer value as the coupling is increased or the photon energy is varied. The subbands show a complex Rabi anticrossing behavior when the photon energy and the coupling bring subbands into resonances. The complicated energy subband structure leads to photon density variations in reciprocal space when resonances occur in the spectrum. The electron-photon coupling polarizes the charge density and tends to reduce the Coulomb exchange effects as the coupling strength increases.

4

Tuning of paramagnetic and diamagnetic cavity photon excitations in a square array of quantum dots in a magnetic field

Gudmundsson, V; Mughnetsyan, V; Goan, HS; Chai, JD; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

NOV 12 2024, PHYSICAL REVIEW B, 110, 205301

DOI: 10.1103/PhysRevB.110.205301

Show abstract

We employ a "real-time" excitation scheme to calculate the excitation spectra of a two-dimensional electron system in a square array of quantum dots placed in a circular cylindrical far-infrared photon cavity subjected to a perpendicular homogeneous external magnetic field. The Coulomb interaction of the electrons is handled via spin density functional theory and the para- and the diamagnetic parts of the electron-photon coupling are updated according to a configuration interaction method in each iteration of the density functional calculation. The results show that an excitation scheme built on using the symmetry of the lateral square superlattice of the dots and the cylindrical cavity produces both para- and diamagnetic resonance peaks with oscillator strengths that can be steered by the excitation pulse parameters. The excitation method breaks the conditions for the generalized Kohn theorem and allows for insight into the subband structure of the electron system and can be used both inside and outside the linear response regime.

5 Open Access

Controlling the excitation spectrum of a quantum dot array with a photon cavity

Gudmundsson, V; Mughnetsyan, V; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

SEP 13 2023, PHYSICAL REVIEW B, 108, 115306

DOI: 10.1103/PhysRevB.108.115306

Show abstract

We use a recently proposed quantum electrodynamical density theory functional in a real-time excitation calculation for a two-dimensional electron gas in a square array of quantum dots in an external constant perpendicular magnetic field to model the influence of cavity photons on the excitation spectra of the system. The excitation is generated by a short electrical pulse. The quantum dot array is defined in an AlGaAs-GaAs heterostructure, which is in turn embedded in a parallel plate far-infrared photon microcavity. The required exchange and correlation energy functionals describing the electron-electron and electron-photon interactions have therefore been adapted for a two-dimensional electron gas in a homogeneous external magnetic field. We predict that the energies of the excitation modes activated by the pulse are generally redshifted to lower values in the presence of a cavity. The redshift can be understood in terms of the polarization of the electron charge by the cavity photons and depends on the magnetic flux, the number of electrons in a unit cell of the lattice, and the electron-photon interaction strength. We find an interesting interplay of the exchange forces in a spin-polarized two-dimensional electron gas and the square-lattice structure leading to a small but clear blueshift of the excitation mode spectra when one electron resides in each dot.

6

Climbing the anisotropy barrier of single-molecule magnets with spin-vibron interaction

Moldoveanu, V; Dragomir, R

JUL 20 2023, PHYSICAL REVIEW B, 108, 024416

DOI: 10.1103/PhysRevB.108.024416

Show abstract

Using the master equation approach, we look for fingerprints of the interaction between the localized spin S of a nanomagnet coupled to spin-polarized leads and its quantized vibrational modes. We find that the stationary and transient currents are sensitive to vibron-assisted transitions of the molecular spin on both sides of the anisotropy barrier. Such transitions are associated with vibron-dressed states and triggered under resonant conditions. Transport calculations are presented for two antiparallel configurations of the spin-polarized electrodes. In the first configuration, and far from a resonance point, a blockade is imposed on both the electronic and molecular spins via their exchange interaction. When sweeping the magnetic field through resonance, the spin-vibron interaction removes this blockade and allows the indirect reading of resonant transitions as the molecular spin climbs the left side of the anisotropy barrier. In the second configuration, the anisotropy barrier is overcome but the vibron-assisted transitions on the right side of the anisotropy barrier "delocalize" the molecular spin and do not allow the complete current-induced magnetic switching -S & RARR; S. In both configurations, the stationary current increases on resonance, due to additional transport channels triggered by the spin-vibron coupling. Therefore, the switching of the spin-vibron coupling could be detected in future transport experiments.

7

Resistive-like Behavior of Ferroelectric p-n Bilayer Structures Based on Epitaxial Pb(Zr0.2Ti0.8)O3 Thin Films

Boni, AG; Chirila, C; Trupina, L; Radu, C; Filip, LD; Moldoveanu, V; Pintilie, I; Pintilie, L

2023 JAN 25 2023, ACS APPLIED ELECTRONIC MATERIALS

DOI: 10.1021/acsaelm.2c01497

Show abstract

The p-n junctions are the building blocks of nowadays electronic devices. The n- or p-type conductivity is obtained in classic semiconductors, like Si, by doping with atoms acting as donors or acceptors, respectively. Doping was used in ferroelectrics to influence the transition temperature, magnitude of some physical properties, but not necessarily conduction type. Therefore, comprehensive studies to obtain true ferroelectric p-n junctions by controlled doping are missing. Recently, it has been shown that Pb(Zr0.2Ti0.8)O-3 films doped with & AP;1% atomic Nb (n-type doping) or Fe (p-type doping) have different orientations of polarization in the as-grown state. Knowing that polarization orientation depends on doping type, the next step is to build ferroelectric p-n homojunctions and to study their properties in relation to ferroelectric polarization. p-n and n-p structures were grown for this purpose by successive deposition of Nb-doped and Fe-doped Pb(Zr,Ti)O-3 layers with different thicknesses. We find that these p-n homojunctions are ferroelectric, but the magnitude of the polarization and coercive field, as well as the dominant polarization orientation in the as-grown state, depend on the conduction type of the first grown layer. The I-V characteristics are quasi-linear, although the interfaces with the electrodes behaves as Schottky contacts. The resistance extracted from the I-V characteristics displays an exponential dependence on temperature, with an activation energy in the range of 0.14-0.17 eV. These results are explained assuming that the total current in the junction is the total of electron and hole injections at the electrode interfaces. It is shown that for relatively low doping concentrations, the current density contains a dominant term with a linear voltage dependence and an exponential temperature dependence, as observed experimentally, and a secondary (correction) term that is dependent on the free carrier density and can induce non-linear voltage dependence when this density is significant.

8 Open Access

Unified approach to cyclotron and plasmon resonances in a periodic two-dimensional GaAs electron gas hosting the Hofstadter butterfly

Gudmundsson, V; Mughnetsyan, V; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

APR 7 2022, PHYSICAL REVIEW B, 105, 155302

DOI: 10.1103/PhysRevB.105.155302

Show abstract

We present theoretical calculations for the cyclotron resonance and various magnetoplasmon modes of a Coulomb interacting two-dimensional GaAs electron gas (2DEG) modulated as a lateral superlattice of quantum dots subjected to an external perpendicular constant magnetic field. We use a real-time excitation approach based on the Liouville???von Neumann equation for the density operator, that can go beyond linear response delivering information of all longitudinal and transverse collective modes of interest to the same order. We perform an extensive analysis of the coexisting collective modes due to the lateral confinement and the magnetic field for a different number of electrons in each dot. In the limit of vanishing dot modulation of the 2DEG we find signs of the structure of the Hofstadter butterfly in the excitation spectra.

9 Open Access

Effects of a far-infrared photon cavity field on the magnetization of a square quantum dot array

Gudmundsson, V; Mughnetsyan, V; Abdullah, NR; Tang, CS; Moldoveanu, V; Manolescu, A

SEP 26 2022, PHYSICAL REVIEW B, 106, 115308

DOI: 10.1103/PhysRevB.106.115308

Show abstract

The orbital and spin magnetization of a cavity-embedded quantum dot array defined in a GaAs heterostruc-ture are calculated within quantum-electrodynamical density-functional theory. To this end, a gradient-based exchange-correlation functional recently employed for atomic systems is adapted to the hosting two-dimensional electron gas submitted to an external perpendicular homogeneous magnetic field. Numerical results reveal the polarizing effects of the cavity photon field on the electron charge distribution and nontrivial changes of the orbital magnetization. We discuss its intertwined dependence on the electron number in each dot, and on the electron-photon coupling strength. In particular, the calculated dispersion of the photon-dressed electron states around the Fermi energy as a function of the electron-photon coupling strength indicates the formation of magnetoplasmon-polaritons in the dots.

10

Spin-vibron coupling effects in single-molecule magnets grafted to a nanoelectromechanical system

Moldoveanu, V; Dragomir, R

AUG 23 2021, PHYSICAL REVIEW B, 104, 075441

DOI: 10.1103/PhysRevB.104.075441

Show abstract

We present a theoretical analysis of the interplay between the spin-vibron and electron-vibron interactions in a hybrid system made of a single-molecule magnet and a suspended conductor. The latter is coupled to particle reservoirs and supports quantized vibrational modes which, once activated, interact with the localized magnetic moment S of the nanomagnet. The dynamics of the molecular spin, the average vibron number, and the transient currents are calculated from the reduced density operator of the hybrid system. We focus on the effect of the vibron-assisted transitions from the lowest energy spin doublet S-z = +/- S to higher energy excited states. The numerical simulations performed for the simplest case S = 2 prove that the vibron-assisted spin transitions and dynamics can be described in terms of a three-level Lambda model borrowed from quantum optics. In particular we predict the existence of Rabi oscillations of the transient currents as fingerprints of the spin-vibron coupling. The role of symmetric or asymmetric bias configurations in setting different mixtures of molecular spin states in the steady-state regime is also emphasized.

11 Open Access

Self-induction and magnetic effects in electron transport through a photon cavity

Gudmundsson, V; Abdullah, NR; Tang, CS; Manolescu, A; Moldoveanu, V

MAR 2021, PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 127, 114544

DOI: 10.1016/j.physe.2020.114544

Show abstract

We explore higher order dynamical effects in the transport through a two-dimensional nanoscale electron system embedded in a three-dimensional far-infrared photon cavity. The nanoscale system is considered to be a short quantum wire with a single circular quantum dot defined in a GaAs heterostructure. The whole system, the external leads and the central system are placed in a constant perpendicular magnetic field. The Coulomb interaction of the electrons, the paraand diamagnetic electron-photon interactions are all treated by a numerically exact diagonalization using step-wise truncations of the appropriate many-body Fock spaces. We focus on the difference in transport properties between a description within an electric dipole approximation and a description including all higher order terms in a single photon mode model. We find small effects mostly caused by an electrical quadrupole and a magnetic dipole terms that depend strongly on the polarization of the cavity field with respect to the transport direction and the photon energy. When the polarization is aligned along the transport direction we find indications of a weak self-induction that we analyze and compare to the classical counterpart, and the self-energy contribution of high-order interaction terms to the states the electrons cascade through on their way through the system. Like expected the electron-photon interaction is well described in the dipole approximation when it is augmented by the lowest order diamagnetic part for a nanoscale system in a cavity in an external magnetic field.

12 Open Access

Quantum turnstile regime of nanoelectromechanical systems

Dragomir, R; Moldoveanu, V; Stanciu, S; Tanatar, B

APR 7 2020, PHYSICAL REVIEW B, 101, 165409

DOI: 10.1103/PhysRevB.101.165409

Show abstract

The effects of a turnstile operation on the current-induced vibron dynamics in nanoelectromechanical systems (NEMS) are analyzed in the framework of the generalized master equation. In our simulations each turnstile cycle allows the pumping of up to two interacting electrons across a biased mesoscopic subsystem which is electrostatically coupled to the vibrational mode of a nanoresonator. The time-dependent mean vibron number is very sensitive to the turnstile driving, rapidly increasing/decreasing along the charging/discharging sequences. This sequence of heating and cooling cycles experienced by the nanoresonator is due to specific vibron-assisted sequential tunneling processes along a turnstile period. At the end of each charging/discharging cycle the nanoresonator is described by a linear combination of vibron-dressed states s(v). associated to an electronic configuration nu. If the turnstile operation leads to complete electronic depletion the nanoresonator returns to its equilibrium position, i.e., its displacement vanishes. It turns out that a suitable bias applied on the NEMS leads to a slow but complete cooling at the end of the turnstile cycle. Our calculations show that the quantum turnstile regime switches the dynamics of the NEMS between vibron-dressed subspaces with different electronic occupation numbers. We predict that the turnstile control of the electron-vibron interaction induces measurable changes on the input and output transient currents.

13

A Dyson Equation for Non-Equilibrium Green's Functions in the Partition-Free Setting

Cornean, HD; Moldoveanu, V; Pillet, CA

JUL 2019, PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 256

DOI: 10.1002/pssb.201800447

Show abstract

Here a small interacting sample, coupled to several non-interacting leads is considered. Initially, the system is at thermal equilibrium. At some instant t(0) the system is set into the so-called partition-free transport scenario by turning on a bias on the leads. Using the theory of Volterra operators we rigorously formulate a Dyson equation for the retarded Green's function and we establish a closed formula for the associated proper interaction self-energy.

14

Generalized Master Equation Approach to Time-Dependent Many-Body Transport

Moldoveanu, V; Manolescu, A; Gudmundsson, V

AUG 2019, ENTROPY, 21

DOI: 10.3390/e21080731

Show abstract

We recall theoretical studies on transient transport through interacting mesoscopic systems. It is shown that a generalized master equation (GME) written and solved in terms of many-body states provides the suitable formal framework to capture both the effects of the Coulomb interaction and electron-photon coupling due to a surrounding single-mode cavity. We outline the derivation of this equation within the Nakajima-Zwanzig formalism and point out technical problems related to its numerical implementation for more realistic systems which can neither be described by non-interacting two-level models nor by a steady-state Markov-Lindblad equation. We first solve the GME for a lattice model and discuss the dynamics of many-body states in a two-dimensional nanowire, the dynamical onset of the current-current correlations in electrostatically coupled parallel quantum dots and transient thermoelectric properties. Secondly, we rely on a continuous model to get the Rabi oscillations of the photocurrent through a double-dot etched in a nanowire and embedded in a quantum cavity. A many-body Markovian version of the GME for cavity-coupled systems is also presented.

15

Cavity-Photon-Induced High-Order Transitions between Ground States of Quantum Dots

Gudmundsson, V; Abdullah, NR; Tang, CS; Manolescu, A; Moldoveanu, V

NOV 2019, ANNALEN DER PHYSIK, 531

DOI: 10.1002/andp.201900306

Show abstract

It is shown that quantum electromagnetic transitions to high orders are essential to describe the time-dependent path of a nanoscale electron system in a Coulomb blockade regime when coupled to external leads and placed in a 3D rectangular photon cavity. The electronic system consists of two quantum dots embedded asymmetrically in a short quantum wire. The two lowest in energy spin degenerate electron states are mostly localized in each dot with only a tiny probability in the other dot. In the presence of the leads, a slow high-order transition between the ground states of the two quantum dots is identified. The Fourier power spectrum for photon-photon correlations in the steady state shows a Fano type of resonance for the frequency of the slow transition. Full account is taken of the geometry of the multilevel electronic system, and the electron-electron Coulomb interactions together with the para- and diamagnetic electron-photon interactions are treated with step-wise exact numerical diagonalization and truncation of appropriate many-body Fock spaces. The matrix elements for all interactions are computed analytically or numerically exactly.

16

Coexisting spin and Rabi oscillations at intermediate time regimes in electron transport through a photon cavity

Gudmundsson, V; Gestsson, H; Abdullah, NR; Tang, CS; Manolescu, A; Moldoveanu, V

MAR 1 2019, BEILSTEIN JOURNAL OF NANOTECHNOLOGY, 10, 616

DOI: 10.3762/bjnano.10.61

Show abstract

In this work, we theoretically model the time-dependent transport through an asymmetric double quantum dot etched in a two-dimensional wire embedded in a far-infrared (FIR) photon cavity. For the transient and the intermediate time regimes, the current and the average photon number are calculated by solving a Markovian master equation in the dressed-states picture, with the Coulomb interaction also taken into account. We predict that in the presence of a transverse magnetic field the interdot Rabi oscillations appearing in the intermediate and transient regime coexist with slower non-equilibrium fluctuations in the occupation of states for opposite spin orientation. The interdot Rabi oscillation induces charge oscillations across the system and a phase difference between the transient source and drain currents. We point out a difference between the steady-state correlation functions in the Coulomb blocking and the photon-assisted transport regimes.

17

Backaction effects in cavity-coupled quantum conductors

Moldoveanu, V; Dinu, IV; Manolescu, A; Gudmundsson, V

SEP 12 2019, PHYSICAL REVIEW B, 100

DOI: 10.1103/PhysRevB.100.125416

Show abstract

We study the electronic transport through a pair of distant nanosystems (S-a and S-b) embedded in a single-mode cavity. Each system is connected to source and drain particle reservoirs and the electron-photon coupling is described by the Tavis-Cummings model. The generalized master equation approach provides the reduced density operator of the double system in the dressed-states basis. It is shown that the photon-mediated coupling between the two subsystems leaves a signature on their transient and steady-state currents. In particular, a suitable bias applied on subsystem S-b induces a photon-assisted current in the other subsystem S-a which is otherwise in the Coulomb blockade. We also predict that a transient current passing through one subsystem triggers a charge transfer between the optically active levels of the second subsystem even if the latter is not connected to the leads. As a result of backaction, the transient current through the open system develops Rabi oscillations (ROs) whose period depends on the initial state of the closed system.

18

Interaction and Size Effects in Open Nano-Electromechanical Systems

Tanatar, B; Moldoveanu, V; Dragomir, R; Stanciu, S

JUN 2019, PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 256

DOI: 10.1002/pssb.201800443

Show abstract

The time-dependent transport of a 2D quantum wire (QW) connected to source/drain leads and electrostatically coupled to a singly-clamped InAs cantilever is investigated. The latter is placed above the nanowire and acts as a nanoresonator (NR) in the quantum regime. The vibron dynamics and the transport properties of this nano-electromechanical system (NEMS) are described within a generalized master equation approach which is exact with respect to the electron-vibron coupling. A detailed description of the electron-vibron coupling by taking into account its dependence on the wavefunctions of the quantum nanowire is introduced. It is shown that the tunneling processes in the QW trigger periodic oscillations of the average vibron number even in the absence of a bias. The time-dependent filling of the vibronic states changes as the nanoresonator is swept along the quantum wire.

19

Many-body effects in transport through a quantum-dot cavity system

Dinu, IV; Moldoveanu, V; Gartner, P

MAY 25 2018, PHYSICAL REVIEW B, 97

DOI: 10.1103/PhysRevB.97.195442

Show abstract

We theoretically describe electric transport through an optically active quantum dot embedded in a single-mode cavity, and coupled to source-drain particle reservoirs. The populations of various many-body configurations (e.g., excitons, trions, biexciton) and the photon-number occupancies are calculated from a master equation which is derived in the basis of dressed states. These take into account both the Coulomb and the light-matter interaction. The former is essential in the description of the transport, while for the latter we identify situations in which it can be neglected in the expression of tunneling rates. The fermionic nature of the particle reservoirs plays an important role in the argument. The master equation is numerically solved for the s-shell many-body configurations of disk-shaped quantum dots. If the cavity is tuned to the biexciton-exciton transition, the most efficient optical processes take place in a three-level A system. The alternative exciton-ground-state route is inhibited as nonresonant due to the biexciton binding energy. The steady-state current is analyzed as a function of the photon frequency and the coupling to the leads. An unexpected feature appears in its dependence on the cavity loss rate, which turns out to be nonmonotonic.

20

A Mathematical Account of the NEGF Formalism

Cornean, HD; Moldoveanu, V; Pillet, CA

FEB 2018, ANNALES HENRI POINCARE, 19, 442

DOI: 10.1007/s00023-017-0638-2

Show abstract

The main goal of this paper is to put on solid mathematical grounds the so-called non-equilibrium Green's function transport formalism for open systems. In particular, we derive the Jauho-Meir-Wingreen formula for the time-dependent current through an interacting sample coupled to non-interacting leads. Our proof is non-perturbative and uses neither complex-time Keldysh contours nor Langreth rules of 'analytic continuation.' We also discuss other technical identities (Langreth, Keldysh) involving various many-body Green's functions. Finally, we study the Dyson equation for the advanced/retarded interacting Green's function and we rigorously construct its (irreducible) self-energy, using the theory of Volterra operators.

21

Unpinning of heavy hole spin in magnetic quantum dots

Dinu, IV; Moldoveanu, V; Dragomir, R; Tanatar, B

MAY 2017, PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 254

DOI: 10.1002/pssb.201600800

Show abstract

Using the kp theory and configuration interaction method, we analyze the effect of heavy hole-light hole (HH-LH) mixing in CdTe quantum dots (QDs) with a single manganese (Mn) ion. We find that the hole-Mn exchange switches the coupling between two excitons whose Luttinger spinors have both HH and LH components. If the magnetic dopant is off-centered and the QD is subjected to a single pulse the system periodically bounces between bright and dark mostly HH excitons with opposite HH spins. A pump-and-probe setup allows to estimate the efficiency of this HH spin unpinning from the biexciton response. The biexciton absorption spectrum is also discussed.

22

Light-hole exciton mixing and dynamics in Mn-doped quantum dots

Moldoveanu, V; Dinu, IV; Dragomir, R; Tanatar, B

APR 18 2016, PHYSICAL REVIEW B, 93

DOI: 10.1103/PhysRevB.93.165421

Show abstract

We investigate theoretically the spectral and dynamical effects of the short-range exchange interaction between a single manganese (Mn) atom hosted by cylindrical CdTe quantum dots and its light-hole excitons or biexcitons. Our approach is based on the Kohn-Luttinger k . p theory and configuration interaction method, the dynamics of the system in the presence of intraband relaxation being derived from the von Neumann-Lindblad equation. The complex structure of the light-hole exciton absorption spectrum reveals the exchange-induced exciton mixing and depends strongly on the Mn position. In particular, if the Mn atom is closer to the edges of the cylinder, the bright and dark light-hole excitons are mixed by the hole-Mn exchange alone. Consequently, their populations exhibit exchange-induced Rabi oscillations which can be viewed as optical signatures of light-hole spin reversal. Similar results are obtained for mixed biexcitons, in this case the exchange-induced Rabi oscillations being damped by the intraband hole relaxation processes. The effect of light-hole heavy-hole mixing is also discussed.

23

Non-equilibrium transport and spin dynamics in single-molecule magnets

Moldoveanu, V; Dinu, IV; Tanatar, B

NOV 2015, SUPERLATTICES AND MICROSTRUCTURES, 87, 76

DOI: 10.1016/j.spmi.2015.06.027

Show abstract

The time-dependent transport through single-molecule magnets (5MM) coupled to magnetic or non-magnetic electrodes is studied in the framework of the generalized Master equation (GME) method. We calculate the transient currents which develop when the molecule is smoothly coupled to the source and drain electrodes. The signature of the electrically induced magnetic switching on these transient currents is investigated. Our simulations show that the magnetic switching of the molecular spin can be read indirectly from the transient currents if one lead is magnetic and it is much faster if the leads have opposite spin polarizations. We identify effects of the transverse anisotropy on the dynamics of molecular states. (C) 2015 Elsevier Ltd. All rights reserved.

24

Quantum turnstile operation of single-molecule magnets

Moldoveanu, V; Dinu, IV; Tanatar, B; Moca, CP

AUG 11 2015, NEW JOURNAL OF PHYSICS, 17

DOI: 10.1088/1367-2630/17/8/083020

Show abstract

The time-dependent transport through single-molecule magnets coupled to magnetic or nonmagnetic electrodes is studied in the framework of the generalized master equation method. We investigate the transient regime induced by the periodic switching of the source and drain contacts. If the electrodes have opposite magnetizations the quantum turnstile operation allows the stepwise writing of intermediate excited states. In turn, the transient currents provide a way to read these states. Within our approach we take into account both the uniaxial and transverse anisotropy. The latter may induce additional quantum tunneling processes which affect the efficiency of the proposed read-and-write scheme. An equally weighted mixture of molecular spin states can be prepared if one of the electrodes is ferromagnetic.

25

INTRABAND RELAXATION OF p-SHELL EXCITONS IN DISK-SHAPED QUANTUM DOTS

Dragomir, R; Moldoveanu, V; Dinu, IV

2015, ROMANIAN JOURNAL OF PHYSICS, 60, 690

Show abstract

We study the generation of p-shell excitons in optically active disk-shaped quantum dots subjected to ultrafast optical pulses. The single-particle spectral properties are obtained from the four-band kp theory, whereas the Coulomb interaction is taken into account within the configuration-interaction approach, particular attention being payed to configuration mixing due to electron-hole correlations. The effect of intraband relaxation processes is included in the non-unitary dynamics derived from the von-Neumann Lindblad equation. We find that the fast hole relaxation processes drive the p-shell excitons to intermediate states which eventually evolve to s-shell excitons via slower electron relaxation.

26

Dynamics and relaxation of sp biexcitons in disk-shaped quantum dots

Moldoveanu, V; Dinu, IV; Dragomir, R

JUN 12 2014, PHYSICAL REVIEW B, 89

DOI: 10.1103/PhysRevB.89.245415

Show abstract

We study the effects of intraband relaxation processes on optical manipulation protocols for sp biexcitons hosted by CdTe disk-shaped quantum dots. The many-body states are calculated within the configuration interaction method starting from single-particle states given by the k.p theory. The time-dependent occupations of relevant many-body states are extracted from the von Neumann-Lindblad equation for the density operator. We mainly investigate the generation of sp biexcitons with two pulses of different polarizations sigma(+) and sigma(-). The fast hole relaxation processes prevent a high-fidelity controlled operation on sp biexcitons and lead to the occupation of some transient states which can be optically probed. More importantly, the many-body structure of the transient states consists of two holes on the s shell and antiparallel sp triplet states for electrons. Our simulations show that these triplet states are more stable against decoherence as they can only be damaged through slow electron relaxation. The configuration mixing due to correlation effects is also discussed.

27

On the Steady State Correlation Functions of Open Interacting Systems

Cornean, HD; Moldoveanu, V; Pillet, CA

OCT 2014, COMMUNICATIONS IN MATHEMATICAL PHYSICS, 331, 295

DOI: 10.1007/s00220-014-1925-0

Show abstract

We address the existence of steady state Green-Keldysh correlation functions of interacting fermions in mesoscopic systems for both the partitioning and partition-free scenarios. Under some spectral assumptions on the non-interacting model and for sufficiently small interaction strength, we show that the system evolves to a NESS which does not depend on the profile of the time-dependent coupling strength/bias. For the partitioned setting we also show that the steady state is independent of the initial state of the inner sample. Closed formulae for the NESS two-point correlation functions (Green-Keldysh functions), in the form of a convergent expansion, are derived. In the partitioning approach, we show that the 0(th) order term in the interaction strength of the charge current leads to the Landauer-Buttiker formula, while the 1(st) order correction contains the mean-field (Hartree-Fock) results.

28

Transport in a hybrid normal metal/topological superconductor Kondo model

Chirla, R; Dinu, IV; Moldoveanu, V; Moca, CP

NOV 5 2014, PHYSICAL REVIEW B, 90

DOI: 10.1103/PhysRevB.90.195108

Show abstract

We investigate the equilibrium and nonequilibrium transport through a quantum dot in the Kondo regime, embedded between a normal metal and a topological superconductor supportingMajorana bound states at its end points. We find that the Kondo physics is significantly modified by the presence of theMajorana modes. When the Majorana modes are coupled, aside from the Kondo scale T-K, a new energy scale T* <> T-K, the regular logarithmic dependence in the differential conductance is also affected. Under nonequilibrium conditions, and in particular in the {T, B}-> 0 limit, the differential conductance becomes negative. These findings indicate that the changes in transport may serve as clues for detecting the Majorana bound states in such systems. In terms of methods used, we characterize the transport by using a combination of perturbative and renormalization-group approaches.

29

Excitation of collective modes in a quantum flute

Torfason, K; Manolescu, A; Moldoveanu, V; Gudmundsson, V

JUN 14 2012, PHYSICAL REVIEW B, 85

DOI: 10.1103/PhysRevB.85.245114

Show abstract

We use a generalized master equation (GME) formalism to describe the nonequilibrium time-dependent transport of Coulomb interacting electrons through a short quantum wire connected to semi-infinite biased leads. The contact strength between the leads and the wire is modulated by out-of-phase time-dependent potentials that simulate a turnstile device. We explore this setup by keeping the contact with one lead at a fixed location at one end of the wire, whereas the contact with the other lead is placed on various sites along the length of the wire. We study the propagation of sinusoidal and rectangular pulses. We find that the current profiles in both leads depend not only on the shape of the pulses, but also on the position of the second contact. The current reflects standing waves created by the contact potentials, like in a wind musical instrument (for example, a flute), but occurring on the background of the equilibrium charge distribution. The number of electrons in our quantum "flute" device varies between two and three. We find that for rectangular pulses the currents in the leads may flow against the bias for short time intervals, due to the higher harmonics of the charge response. The GME is solved numerically in small time steps without resorting to the traditional Markov and rotating wave approximations. The Coulomb interaction between the electrons in the sample is included via the exact diagonalization method. The system (leads plus sample wire) is described by a lattice model.

30

Analysis of the phase lapse problem in closed interferometers

Tolea, M; Moldoveanu, V; Dinu, IV; Tanatar, B

OCT 1 2012, PHYSICS LETTERS A, 376, 3234

DOI: 10.1016/j.physleta.2012.07.007

Show abstract

We investigate the connection between the asymmetry of the Fano resonances in a mesoscopic interferometer with an embedded quantum dot and the pi lapses in the phase of the "bare" dot transmittance. Consecutive Fano resonances with the same (opposite) sign of the Fano parameter imply the presence (absence) of a phase lapse with pi between the corresponding resonances of the dot. Our results suggest that the famous "phase lapse" problem, first reported by Schuster et al. [R. Schuster, E. Buks, M. Heiblum, D. Mahalu, V. Umansky, H. Shtrikman, Nature 385 (1997) 417], can therefore be experimentally addressed in closed interferometers. It is also proposed that the Fano effect can be used to extract the phase distributions of the eigenfunctions for a mesoscopic 20 shape, via the parity of the resonances. In the presence of electron-electron interaction, one can calculate the phases of the T-matrix elements. The numerical results lead to the same conclusions as for the non-interacting case. (C) 2012 Elsevier B.V. All rights reserved.

31

Electronic transmittance phase extracted from mesoscopic interferometers

Tolea, M; Moldoveanu, V; Dinu, IV; Tanatar, B

OCT 13 2012, NANOSCALE RESEARCH LETTERS, 7, 7

DOI: 10.1186/1556-276X-7-568

Show abstract

The usual experimental set-up for measuring the wave function phase shift of electrons tunneling through a quantum dot (QD) embedded in a ring (i.e., the transmittance phase) is the so-called 'open' interferometer as first proposed by Schuster et al. in 1997, in which the electrons back-scattered at source and the drain contacts are absorbed by additional leads in order to exclude multiple interference. While in this case one can conveniently use a simple two-path interference formula to extract the QD transmittance phase, the open interferometer has also a number of draw-backs, such as a reduced signal and some uncertainty regarding the effects of the extra leads. Here we present a meaningful theoretical study of the QD transmittance phase in 'closed' interferometers (i.e., connected only to source and drain leads). By putting together data from existing literature and giving some new proofs, we show both analytically and by numerical simulations that the existence of phase lapses between consecutive resonances of the 'bare' QD is related to the signs of the corresponding Fano parameters - of the QD + ring system. More precisely, if the Fano parameters have the same sign, the transmittance phase of the QD exhibits a I lapse. Therefore, closed mesoscopic interferometers can be used to address the 'universal phase lapse' problem. Moreover, the data from already existing Fano interference experiments from Kobayashi et al. in 2003 can be used to infer the phase lapses.

32

Mesoscopic Fano effect in a spin splitter with a side-coupled quantum dot

Moldoveanu, V; Tolea, M; Tanatar, B

FEB 20 2012, PHYSICS LETTERS A, 376, 1083

DOI: 10.1016/j.physleta.2012.02.017

Show abstract

We investigate the interplay between the spin interference and the Fano effect in a three-lead mesoscopic ring with a side-coupled quantum dot (QD). A uniform Rashba spin-orbit coupling and a perpendicular magnetic field are tuned such that the ring operates as a spin splitter in the absence of the QD: one lead is used to inject unpolarized electrons and the remaining (output) leads collect almost polarized spin currents. By applying a gate potential to the quantum dot a pair of spin-split levels sweeps the bias window and leads to Fano interference. The steady-state spin and charge currents in the leads are calculated for a finite bias applied across the ring via the non-equilibrium Green's function formalism. When the QD levels participate to transport we find that the spin currents exhibit peaks and dips whereas the charge currents present Fano lineshapes. The location of the side-coupled quantum dot and the spin splitting of its levels also affect the interference and the output currents. The opposite response of output currents to the variation of the gate potential allows one to use this system as a single parameter current switch. We also analyze the dependence of the splitter efficiency on the spin splitting on the QD. (C) 2012 Elsevier B.V. All rights reserved.

33

Nonequilibrium steady states for interacting open systems: Exact results

Moldoveanu, V; Cornean, HD; Pillet, CA

AUG 11 2011, PHYSICAL REVIEW B, 84

DOI: 10.1103/PhysRevB.84.075464

Show abstract

Under certain conditions, we prove the existence of a steady-state transport regime for interacting mesoscopic systems coupled to reservoirs (leads). The partitioning and partition-free scenarios are treated on an equal footing. Our time-dependent scattering approach is exact and proves, among other things, the independence of the steady-state quantities from the initial state of the sample. Closed formulas for the steady-state current amenable for perturbative calculations with regard to the interaction strength are also derived. In the partitioning case, we calculate the first-order correction and recover the mean-field (Hartree-Fock) results.

34

Turnstile pumping through an open quantum wire

Gainar, CM; Moldoveanu, V; Manolescu, A; Gudmundsson, V

JAN 2011, NEW JOURNAL OF PHYSICS, 13

DOI: 10.1088/1367-2630/13/1/013014

Show abstract

We use a non-Markovian generalized master equation (GME) to describe the time-dependent charge transfer through a parabolically confined quantum wire of a finite length coupled to semi-infinite quasi-two-dimensional (2D) leads. The quantum wire and the leads are in a perpendicular external magnetic field. The contacts to the left and right leads depend on time and are kept out of phase to model a quantum turnstile of finite size. The effects of the driving period of the turnstile, the external magnetic field, the character of the contacts and the chemical potential bias on the effectiveness of the charge transfer of the turnstile are examined, in both the absence and the presence of the magnetic field. The interplay between the strength of the coupling and the strength of the magnetic field is also discussed. We observe how the edge states created in the presence of the magnetic field contribute to the pumped charge.

35

Time-dependent magnetotransport in semiconductor nanostructures via the generalized master equation

Gudmundsson, V; Tang, CS; Gainar, CM; Moldoveanu, V; Manolescu, A

JAN 2011, COMPUTER PHYSICS COMMUNICATIONS, 182, 48

DOI: 10.1016/j.cpc.2010.08.006

Show abstract

Transport of electrons through two-dimensional semiconductor structures on the nanoscale in the presence of perpendicular magnetic field depends on the interplay of geometry of the system the leads and the magnetic length We use a generalized master equation (GME) formalism to describe the transport through the system without resorting to the Markov approximation Coupling to the leads results in elastic and inelastic processes in the system that are described to a high order by the integro-differential equation of the GME formalism Geometrical details of systems and leads leave their fingerprints on the transport of electrons through them The GME formalism can be used to describe both the initial transient regime immediately after the coupling of the leads to the system and the steady state achieved after a longer time (C) 2010 Elsevier BV All rights reserved

36

On the cotunneling regime of interacting quantum dots

Cornean, HD; Moldoveanu, V

JUL 29 2011, JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL, 44

DOI: 10.1088/1751-8113/44/30/305002

Show abstract

Consider a bunch of interacting electrons confined in a quantum dot. The later is suddenly coupled to semi-infinite biased leads at an initial instant t = 0. We identify the dominant contribution to the ergodic current in the off-resonant transport regime, in which the discrete spectrum of the quantum dot is well separated from the absolutely continuous spectrum of the leads. Our approach allows for arbitrary strength of the electron-electron interaction while the current is expanded in even powers of the (weak) lead-dot hopping constant tau. We provide explicit calculations for sequential tunneling and cotunneling contributions to the current. In the interacting case, it turns out that the cotunneling current depends on the initial many-body configuration of the sample, while in the non-interacting case, it does not and coincides with the first term in the expansion of the Landauer formula w.r.t. tau.

37

Current enhancement and negative differential conductance in parallel quantum dot systems

Tanatar, B; Moldoveanu, V

2011, PHYSICS OF SEMICONDUCTORS: 30TH INTERNATIONAL CONFERENCE ON THE PHYSICS OF SEMICONDUCTORS, 1399

DOI: 10.1063/1.3666366

Show abstract

We present calculations on the transport properties of a double quantum dot (DQD) capacitively coupled to another individually biased dot. The effects of the intradot and interdot Coulomb interaction are included within the random-phase approximation (RPA) implemented in the Keldysh formalism. We show that by increasing the bias on the nearby dot the inelastic Coulomb scattering modifies the current in the double dot. The sign of the current depends on the detuning of the double dot levels and intradot transitions lead to negative differential conductance. The enhancement of the current due to the energy quanta transferred from the strongly biased dot suggests a quantum ratchet or Coulomb drag mechanism.

38

Tunable spin currents in a biased Rashba ring

Moldoveanu, V; Tanatar, B

JAN 2010, PHYSICAL REVIEW B, 81

DOI: 10.1103/PhysRevB.81.035326

Show abstract

The effect of Rashba spin-orbit coupling on the spin interference in a noninteracting one-dimensional ring connected to two leads is studied theoretically within the nonequilibrium Greens' function formalism. We compute the charge and spin currents and analyze their Aharonov-Bohm oscillations. The geometry of the system is conveniently described by the angle delta between the two leads. We show that for delta=180 degrees (i.e., for symmetrically coupled leads), a good filtering of up-or down-spin orientation is obtained around half-integer multiples of Phi/Phi(0). These particular flux values are degeneracy points for clockwise and counterclockwise propagating states, corresponding to the same spin orientation in the local spin frame of the ring. In contrast, for the asymmetric coupling, i.e., delta=135 degrees, the filter efficiency is maximum around integer multiples of Phi/Phi(0). The numerical results suggest that the spin filtering is obtained when the clockwise or counterclockwise states interfere destructively. It turns out that the spin filtering regime is stable against variations in the bias applied on the system. The quasiperiodic oscillations of the charge current, as a function of the Rashba strength, are obtained and discussed.

39

Coulomb interaction and transient charging of excited states in open nanosystems

Moldoveanu, V; Manolescu, A; Tang, CS; Gudmundsson, V

APR 15 2010, PHYSICAL REVIEW B, 81

DOI: 10.1103/PhysRevB.81.155442

Show abstract

We obtain and analyze the effect of electron-electron Coulomb interaction on the time-dependent current flowing through a mesoscopic system connected to biased semi-infinite leads. We assume the contact is gradually switched on in time and we calculate the time-dependent reduced density operator of the sample using the generalized master equation. The many-electron states (MES) of the isolated sample are derived with the exact-diagonalization method. The chemical potentials of the two leads create a bias window which determines which MES are relevant to the charging and discharging of the sample and to the currents, during the transient or steady states. We discuss the contribution of the MES with fixed number of electrons N and we find that in the transient regime there are excited states more active than the ground state even for N=1. This is a dynamical signature of the Coulomb-blockade phenomenon. We discuss numerical results for three sample models: short one-dimensional chain, two-dimensional (2D) lattice, and 2D parabolic quantum wire.

40

Correlated time-dependent transport through a two-dimensional quantum structure

Gudmundsson, V; Tang, CS; Jonasson, O; Moldoveanu, V; Manolescu, A

MAY 15 2010, PHYSICAL REVIEW B, 81

DOI: 10.1103/PhysRevB.81.205319

Show abstract

We use a generalized master equation (GME) to describe the nonequilibrium magnetotransport of interacting electrons through a broad finite quantum wire with an embedded ring structure. The finite quantum wire is weakly coupled to two broad leads acting as reservoirs of electrons. The mutual Coulomb interaction of the electrons is described using a configuration interaction method for the many-electron states of the central system. We report some nontrivial interaction effects both at the level of time-dependent filling of states and on the time-dependent transport. We find that the Coulomb interaction in this nontrivial geometry can enhance the correlation of electronic states in the system and facilitate it's charging in certain circumstances in the weak coupling limit appropriate for the GME. In addition, we find oscillations in the current in the leads due to the correlations oscillations caused by the switched-on lead-system coupling. The oscillations are influenced and can be enhanced by the external magnetic field and the Coulomb interaction.

41

Dynamic correlations induced by Coulomb interactions in coupled quantum dots

Moldoveanu, V; Manolescu, A; Gudmundsson, V

AUG 11 2010, PHYSICAL REVIEW B, 82

DOI: 10.1103/PhysRevB.82.085311

Show abstract

Time-dependent transport through two capacitively coupled quantum dots is studied in the framework of the generalized master equation. The Coulomb interaction is included within the exact diagonalization method. Each dot is connected to two leads at different times, such that a steady state is established in one dot before the coupling of the other dot to its leads. By appropriately tuning the bias windows on each dot we find that in the final steady state the transport may be suppressed or enhanced. These two cases are explained by the redistribution of charge on the many-body states built on both dots. We also predict and analyze the transient mutual charge sensing of the dots.

42

Spin splitter regime of a mesoscopic Rashba ring

Moldoveanu, V; Tanatar, B

DEC 1 2010, PHYSICS LETTERS A, 375, 191

DOI: 10.1016/j.physleta.2010.10.047

Show abstract

Using the non-equilibrium Greens' function formalism we calculate the spin currents in a one-dimensional ring coupled to three leads and in the presence of perpendicular magnetic flux (1) and Rashba spin-orbit coupling. A finite bias is applied between the input lead and the other two output leads. We show that the spin-orbit coupling allows one to operate this system as a spin splitter, i.e. the output leads deliver spin-polarized currents with different orientations. We find that the spin splitter operation can be tuned at integer multiples of phi/phi(0). Its efficiency depends not only on the value of the Rashba coupling but also on the bias applied between the input and output leads. The selected spin orientation of the output leads can be reversed by a slight change of their contact position. We discuss as well the connection between the spin splitter operation and the spectral properties of the ring. (C) 2010 Elsevier B.V. All rights reserved.

43

Inelastic transitions and counterflow tunneling in double-dot quantum ratchets

Moldoveanu, V; Tanatar, B

NOV 10 2010, PHYSICAL REVIEW B, 82

DOI: 10.1103/PhysRevB.82.205312

Show abstract

The ratchet regime of unbiased double quantum dots driven out of equilibrium by an independently biased nearby detector has been theoretically studied using the nonequilibrium Keldysh formalism and the random-phase approximation for the Coulomb effects. When the detector is suitably biased the energy exchange between the two systems removes the Coulomb blockade on the double dot via inelastic interdot tunneling. The energy detuning determines whether the current flows in the same direction as the driving current (positive flow) or in the opposite direction (electronic counterflow). In both cases the intradot transitions lead to negative-differential conductance. Besides the ratchet contribution to the current we also single out a Coulomb drag component.

44

RPA APPROACH TO NON-LINEAR TRANSPORT IN QUANTUM DOTS

Tanatar, B; Moldoveanu, V

2010, CONDENSED MATTER THEORIES, VOL 24, +

DOI: 10.1142/9789814289153_0040

Show abstract

An accurate theoretical treatment of electron-electron interactions in mesoscopic systems is available in very few cases and approximation schemes are developed in most of the applications, especially for many-level quantum dots. Here we present transport calculations within the random-phase approximation for the Coulomb interaction using the Keldysh Green's functions formalism. We describe the quantum dot systems by a tight-binding Hamiltonian. Our method is similar to the one used by Faleev and Stockman [Phys. Rev. B 66 085318 (2002)] in their study of the equilibrium properties of a homogeneous 2D electron gas. The important extension at the formal level is that we combine the RPA and the Keldysh formalism for studying non-linear transport properties of open quantum dots. Within the Keldysh formalism the polarization operator becomes a contour-ordered quantity that should be computed either from the non-interacting Green functions of the coupled quantum dot (the so-called G(0)W approximation) either self-consistently (GW approximation). We performed both non-selfconsistent and self-consistent calculations and compare the results. In particular we recover the Coulomb diamonds for interacting quantum dots and we discuss the charge sensing effects in parallel quantum dots.

45

Time-dependent transport via the generalized master equation through a finite quantum wire with an embedded subsystem

Gudmundsson, V; Gainar, C; Tang, CS; Moldoveanu, V; Manolescu, A

NOV 4 2009, NEW JOURNAL OF PHYSICS, 11

DOI: 10.1088/1367-2630/11/11/113007

Show abstract

In this paper, we apply the generalized master equation to analyze time-dependent transport through a finite quantum wire with an embedded subsystem. The parabolic quantum wire and the leads with several subbands are described by a continuous model. We use an approach originally developed for a tight-binding description selecting the relevant states for transport around the bias-window defined around the values of the chemical potential in the left and right leads in order to capture the effects of the nontrivial geometry of the system in the transport. We observe a partial current reflection as a manifestation of a quasi-bound state in an embedded well and the formation of a resonance state between an off-set potential hill and the boundary of the system.

46

Coulomb drag in parallel quantum dots

Moldoveanu, V; Tanatar, B

JUN 2009, EPL, 86

DOI: 10.1209/0295-5075/86/67004

Show abstract

We study theoretically the electronic transport in parallel few-level quantum dots in the presence of both intradot and interdot long-range Coulomb interaction. Each dot is connected to two leads and the steady-state currents are calculated within the Keldysh formalism using the random-phase approximation for the interacting Green functions. Due to the momentum transfer between the two systems it is possible to get a nonvanishing current through an unbiased Coulomb-blockaded dot, if the other dot is set in the nonlinear transport regime. The transitions between the levels of the passive dot reduce the drag current and lead to negative differential conductance. We also discuss the dependence on temperature and the role of the lead-dot coupling. Copyright (C) EPLA, 2009

47

Fano effect in a double T-shaped interferometer

Moldoveanu, V; Dinu, IV; Tanatar, B

JAN 2009, EUROPEAN PHYSICAL JOURNAL B, 67, 238

DOI: 10.1140/epjb/e2009-00012-0

Show abstract

We study the coherent transport in a one-dimensional lead with two side-coupled quantum dots using the Keldysh's Green function formalism.The effect of the interdot Coulomb interaction is taken into account by computing the firstand second order contributions to the self-energy.We show that the Fano interference due to the resonance of one dotis strongly affected by the fixed parameters that characterize the second dot. If the second dot is tuned close to resonance an additionalpeak develops between the peak and dip of the Fano line shape of the current. In contrast, when the second dotis off-resonance and its occupation number is close to unity the interdot Coulomb interaction merely shifts the Fano line and no other maxima appear.The system we consider is more general than the single-dot interferometer studied experimentally by Kobayashi et al. [Phys. Rev. B 70, 035319 (2004)] and may be used for controlling quantum interference and studying decoherence effects in mesoscopic transport.

48

RPA APPROACH TO NON-LINEAR TRANSPORT IN QUANTUM DOTS

Tanatar, B; Moldoveanu, V

AUG 20 2009, INTERNATIONAL JOURNAL OF MODERN PHYSICS B, 23, 4421

DOI: 10.1142/S0217979209063560

Show abstract

An accurate theoretical treatment of electron-electron interactions in mesoscopic systems is available in very few cases and approximation schemes are developed in most of the applications, especially for many-level quantum dots. Here we present transport calculations within the random-phase approximation for the Coulomb interaction using the Keldysh Green's functions formalism. We describe the quantum dot systems by a tight-binding Hamiltonian. Our method is similar to the one used by Faleev and Stockman [Phys. Rev. B 66 085318 (2002)] in their study of the equilibrium properties of a homogeneous 2D electron gas. The important extension at the formal level is that we combine the RPA and the Keldysh formalism for studying non-linear transport properties of open quantum dots. Within the Keldysh formalism the polarization operator becomes a contour-ordered quantity that should be computed either from the non-interacting Green functions of the coupled quantum dot (the so-called G(0)W approximation) either self-consistently (GW approximation). We performed both non-selfconsistent and self-consistent calculations and compare the results. In particular we recover the Coulomb diamonds for interacting quantum dots and we discuss the charge sensing effects in parallel quantum dots.

49

Geometrical effects and signal delay in time-dependent transport at the nanoscale

Moldoveanu, V; Manolescu, A; Gudmundsson, V

JUL 7 2009, NEW JOURNAL OF PHYSICS, 11

DOI: 10.1088/1367-2630/11/7/073019

Show abstract

Nonstationary and steady-state transport through a mesoscopic sample connected to particle reservoirs via time-dependent barriers is investigated by the reduced density operator method. The generalized master equation is solved via the Crank-Nicolson algorithm by taking into account the memory kernel which embodies the non-Markovian effects that are commonly disregarded. The lead-sample coupling takes into account the match between the energy of the incident electrons and the levels of the isolated sample, as well as their overlap at the contacts. Using a tight-binding description of the system, we investigate the effects induced in the transient current by the spectral structure of the sample and by the localization properties of its eigenfunctions. In strong magnetic fields, the transient currents propagate along edge states. The behavior of populations and coherences is discussed, as well as their connection to the tunneling processes that are relevant for transport.

50

Theoretical investigation of modulated currents in open nanostructures

Moldoveanu, V; Manolescu, A; Gudmundsson, V

NOV 2009, PHYSICAL REVIEW B, 80

DOI: 10.1103/PhysRevB.80.205325

Show abstract

We investigate theoretically the transport properties of a mesoscopic system driven by a sequence of rectangular pulses applied at the contact to the input (left) lead. The characteristics of the current which would be measured in the output (right) lead are discussed in relation with the spectral properties of the sample. The time-dependent currents are calculated via a generalized non-Markovian master equation scheme. We study the transient response of a quantum dot and of a narrow quantum wire. We show that the output response depends not only on the lead-sample coupling and on the length of the pulse but also on the states that propagate the input signal. We find that by increasing the bias window the new states available for transport induce additional structure in the relaxation current due to different dynamical tunneling processes. The delay of the output signal with respect to the input current in the case of the narrow quantum wire is associated to the transient time through the wire.

51

Coulomb drag effect in parallel quantum dots

Tanatar, B; Moldoveanu, V

2009, TRANSPORT AND OPTICAL PROPERTIES OF NANOMATERIALS, 1147, +

Show abstract

We study theoretically the electronic transport in parallel few-level quantum dots in the presence of both intradot and interdot long-range Coulomb interaction. Each dot is connected to two leads and the steady-state currents are calculated within the Keldysh formalism using the random-phase approximation for the interacting Green functions. Due to the momentum transfer mechanism between the two systems it is possible to get a nonvanishing current through an unbiased Coulomb-blockaded dot if the other dot is set in the nonlinear transport regime. The transitions between the levels of the passive dot reduce the drag current and lead to negative differential conductance.

52

Transient magnetotransport through a quantum wire

Gudmundsson, V; Thorgilsson, G; Tang, CS; Moldoveanu, V

JAN 2008, PHYSICAL REVIEW B, 77

DOI: 10.1103/PhysRevB.77.035329

Show abstract

We consider an ideal parabolic quantum wire in a perpendicular magnetic field. A simple Gaussian-shaped scattering potential well or hill is flashed softly on and off with its maximum at t=0, mimicking a temporary broadening or narrowing of the wire. By an extension of the Lippmann-Schwinger formalism to time-dependent scattering potentials, we investigate the effects on the continuous current that is driven through the quantum wire with a vanishingly small forward bias. The Lippmann-Schwinger approach to the scattering process enables us to investigate the interplay between geometrical effects and effects caused by the magnetic field.

53

Coherent and incoherent transport through T-shaped double quantum dots

Moldoveanu, V; Tolea, M; Tanatar, B

MAR 2008, PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 40, 1104

DOI: 10.1016/j.physe.2007.08.012

Show abstract

We investigate the measurement induced dephasing of the Fano effect in the electronic transport through a double quantum dot mesoscopic interferometer coupled to a charge detector. The current and the differential conductance are computed within the Keldysh formalism, taking into account of the inelastic processes due to the dot-detector interaction. We show that the visibility of the Fano lineshape is reduced by applying a finite bias on the charge detector. (C) 2007 Elsevier B.V. All rights reserved.

54

Coulomb effects in open quantum dots within the random-phase approximation

Moldoveanu, V; Tanatar, B

MAY 2008, PHYSICAL REVIEW B, 77

DOI: 10.1103/PhysRevB.77.195302

Show abstract

The effect of electron-electron interactions on coherent transport in quantum dot systems is theoretically investigated by adapting the well-known random-phase approximation (RPA) to the nonequilibrium GreenKeldysh formalism for open mesoscopic systems. The contour-ordered polarization operator is computed in terms of the Green functions of the noninteracting system. We apply the proposed RPA-Keldysh scheme for studying Coulomb-modified Fano lines and dephasing effects in interferometers with side-coupled many-level dots. Our method allows us to treat on equal footing the decoherence induced by the intradot interaction and that by the Coulomb coupling to a nearby system. In the case of a single interferometer, we show that the intradot Coulomb interaction leads to a reduction of-the Fano line amplitude. From the analysis of the interaction self-energy, it follows that this effect originates in inelastic scattering processes in which electron-hole pairs are involved. The interplay between the interdot and the intradot interactions in decoherence is discussed for two nearby identical T-shaped interferometers. We also show that the intradot interaction does not prevent the observation of controlled dephasing due to a nearby charge detector, as long as the latter is subjected to a sufficiently large bias.

55

Measurement-induced decoherence in electronic interferometry at nanoscale

Moldoveanu, V; Tanatar, B; Tolea, M

SEP 29 2008, PHYSICS LETTERS A, 372, 6196

DOI: 10.1016/j.physleta.2008.07.079

Show abstract

We introduce a theoretical formalism describing a wide class of 'Which Path' experiments in mesoscopic/nanoscopic transport. The physical system involves a mesoscopic interferometer (e.g. an Aharonov-Bohm ring with embedded dots or a side-coupled quantum dot) which is electrostatically coupled to a nearby quantum point constriction. Due to the charge sensing effect the latter acts as a charge detector. Therefore the interference pattern can be monitored indirectly by looking at the current characteristics of the detector as shown in the experimental work of Buks et al. [E. Buks, R. Schuster, M. Heiblum, D. Mahalu, V. Umansky, Nature (London) 391 (1998) 871]. We use the non-equilibrium Green-Keldysh formalism and a second order perturbative treatment of the Coulomb interaction in order to compute the relevant transport properties. it is shown that in the presence of the Coulomb interaction the current through the detector exhibits oscillations as a function of the magnetic field applied on a single-dot AB interferometer. We also discuss the dependence of the visibility of the Aharonov-Bohm oscillations on the gate potential applied to the dot. (C) 2008 Elsevier B.V. All rights reserved.

56

Controlled dephasing in single-dot Aharonov-Bohm interferometers

Moldoveanu, V; Tolea, M; Tanatar, B

JAN 2007, PHYSICAL REVIEW B, 75

DOI: 10.1103/PhysRevB.75.045309

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We study the Fano effect and the visibility of the Aharonov-Bohm oscillations for a mesoscopic interferometer with an embedded quantum dot in the presence of a nearby second dot. When the electron-electron interaction between the two dots is considered the nearby dot acts as a charge detector. We compute the currents through the interferometer and detector within the Keldysh formalism and the self-energy of the nonequilibrium Green's functions is found up to the second order in the interaction strength. The current formula contains a correction to the Landauer-Buttiker formula. Its contribution to transport and dephasing is discussed. As the bias applied on the detector is increased, the amplitude of both the Fano resonance and Aharonov-Bohm oscillations are considerably reduced due to controlled dephasing. This result is explained by analyzing the behavior of the imaginary part of the interaction self-energy as a function of energy and bias. We emphasize as well the role of the ring-dot coupling. Our theoretical results are consistent with the experimental observation of Buks [Nature 391, 871 (1998)].

57

Nonadiabatic transport in a quantum dot turnstile

Moldoveanu, V; Gudmundsson, V; Manolescu, A

OCT 2007, PHYSICAL REVIEW B, 76

DOI: 10.1103/PhysRevB.76.165308

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We present a theoretical study of the electronic transport through a many-level quantum dot driven by time-dependent signals applied at the contacts to the leads. If the barriers oscillate out of phase, the system operates like a turnstile pump under a finite constant bias, as observed in the experiments of Kouwenhoven [Phys. Rev. Lett. 67, 1626 (1991)]. The time-dependent currents and their averages over successive pumping periods are computed from the Keldysh formalism for tight-binding models. The calculation considers a sudden application of the pumping potentials at t=0, which leads to transient features of the time-dependent and averaged currents during the first pumping cycles which turn out to be important in the high-frequency regime. We show that in the transient regime, the efficiency of the system as a pump is rather poor because it mainly absorbs charge from both leads in order to fill the levels located below the bias window. Under a finite bias and a low-frequency pumping signal, the charge transferred across the system depends on the number of levels located within the bias window. The internal charge dynamics and the role of energy sidebands are investigated. The so-called satellite peaks of the averaged current are also observed in the transient regime.

58

Mesoscopic Fano effect in an Aharonov-Bohm interferometer Coulomb-coupled to a nearby quantum dot

Tolea, M; Moldoveanu, V; Tanatar, B

2007, PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 4, NO 2, 4, +

DOI: 10.1002/pssc.200673304

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Motivated by the pionieering experiments of Buks et al. [Nature 391, 871 (1998)] we investigate the visibility of the Fano effect in a single-dot Aharonov-Bohm interferometer which is Coulomb-coupled to a nearby quantum dot. The latter acts as a 'Which Path Detector' and is coupled to two leads on which a finite bias is applied. Using the non-equilibrium Keldysh-Green function formalism we compute the currents through the detector and the interferometer. We take into account the first two contributions to the interaction self energy and emphasize the correction to the Landauer formula which appears beyond the single-particle approximation. Particular attention is given to the coherence properties of the interferometer in the presence of the electron-electron interaction between the embedded dot and the detector. We show that when the detector is subjected to a finite bias the amplitude of Aharonov-Bohm oscillations of the current through the interferometer decreases. The Fano line is in turn rather stable under interaction. Our results generalize an earlier work of Silva and Levit [Phys. Rev. B 63, 201309 (2001)] and complement the existing description of the controlled dephasing. (c) 2007 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

59

Transient regime in nonlinear transport through many-level quantum dots

Moldoveanu, V; Gudmundsson, V; Manolescu, A

AUG 2007, PHYSICAL REVIEW B, 76

DOI: 10.1103/PhysRevB.76.085330

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We investigate nonstationary electronic transport in noninteracting nanostructures driven by a finite bias and time-dependent signals applied at their contacts to the leads. The systems are modeled by a tight-binding Hamiltonian, and the transient currents are computed from the nonequilibrium Green-Keldysh formalism. The numerical implementation is not restricted to weak coupling to the leads and does not imply the wideband limit assumption for the spectral width of the leads. As an application of the method we study in detail the transient behavior and the charge dynamics in single and double quantum dots connected to leads by a steplike potential, but the method allows as well consideration of nonperiodic potentials or short pulses. We show that when the higher-energy levels of the isolated system are located within the bias window of the leads, the transient current approaches the steady state in a nonoscillatory smooth fashion. At moderate coupling to the leads and fixed bias the transient acquires a steplike structure, the length of the steps increasing with system size. The number of levels inside a finite bias window can be tuned by a constant gate potential. We find also that the transient behavior depends on the specific way of coupling the leads to the mesoscopic system.

60

Mesoscopic Fano effect in Aharonov-Bohm rings with an embedded double dot

Tanatar, B; Moldoveanu, V; Tolea, M; Aldea, A

2006, LOW TEMPERATURE PHYSICS, PTS A AND B, 850, +

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We investigate theoretically in a tight-binding model the transport properties of the Aharonov-Bohm interferometer (ABI) with one dot embedded in each of its arms. For weak interdot coupling the model Hamiltonian describes the system considered in the experiments of Holleitner et al. [Phys. Rev. Lett. 87, 256802 (2001)]. The electronic transmittance of the interferometer is computed within the Landauer-Buttiker formalism while the coexistence of resonant and coherent transport is explicitly emphasized by using the Feschbach formula. The latter produces effective Hamiltonians whose spectral properties describe the tunneling processes through each dot. We reproduce numerically the stability charging diagrams reported in the experiments of Holleitner et al. When the magnetic flux is fixed and one dot is set to resonance the interferometer transmittance shows Fano, lineshapes as a function of the gate voltage applied to the other dot. Our model includes the effect of the magnetic field on the dot levels and explains the change of the asymmetric tail as the magnetic flux is varied. The transmittance assigned to the Fano, dips located in the almost crossing point of the charging diagrams shows Aharonov-Bohm oscillations.

61

Fano interference in mesoscopic rings with quantum dots

Moldoveanu, V; Aldea, A; Tolea, M

2006, PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 3, NO 2, 3, +

DOI: 10.1002/pssc.200562736

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We propose a general formalism for describing the coexistence of coherent and resonant transport in hybrid mesoscopic structures. The approach is based on Landauer- Buttiker formula for the electronic transmittance and on an old formula of Feshbach. The latter gives the complete Green function of coupled subsystems in terms of effective Green functions of the disconnected parts and provides informations about the individual contributions of each subsystem to transport. Motivated by the experiments of Kobayashi et al.(Phys. Rev. Lett. 88, 256806 (2002)) and Holleitner et al. (Phys. Rev. Lett. 87, 256802 (2001)) we apply the formalism to study transport in Aharonov-Bohm interferometers (ABI) containing one or two coupled two-dimensional quantum dots (QD). In the single dot case, we reproduce and explain the magnetic field control of the Fano interference and investigate the interaction effects in a self-consistent approach. In the double dot case, we obtain the charging diagrams and establish precise criteria for the observation of mesoscopic Fano effect and AB oscillations. (c) 2006 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

62

The dynamics of one-dimensional Bloch electrons in constant electric fields

Bentosela, F; Duclos, P; Moldoveanu, V; Nenciu, G

APR 2005, JOURNAL OF MATHEMATICAL PHYSICS, 46

DOI: 10.1063/1.1870732

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We study the dynamics of a one-dimensional Bloch electron subjected to a constant electric field. The periodic potential is supposed to be less singular than the delta-like potential (Dirac comb). We give a rigorous proof of Ao's result that for a large class of initial conditions (high momentum regime) there is no localization in momentum space. The proof is based on the mathematical substantiation of the two simplifying assumptions made in physical literature: the transitions between far away bands can be neglected and the transitions at the quasicrossing can be described by Landau-Zener-type formulas. Using the connection between the above model and the driven quantum ring (DQR) shown by Avron and Nemirovski, our results imply the increase of energy for weakly singular such DQR and appropiate initial conditions. (C) 2005 American Institute of Physics.

63

Fano regime of one-dot Aharonov-Bohm interferometers

Moldoveanu, V; Tolea, M; Gudmundsson, V; Manolescu, A

AUG 2005, PHYSICAL REVIEW B, 72

DOI: 10.1103/PhysRevB.72.085338

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We use the Landauer-Buttiker formalism to study the mesoscopic Fano effect in Aharonov-Bohm rings with an embedded two-dimensional noninteracting dot. The magnetic field dependence of the dot levels leads to a global shift of the Fano lines which becomes important for small ring/dot area ratios. As the magnetic field is varied the Fano dips move periodically from one side of the peak to the other, as reported by Kobayashi [Phys. Rev. Lett. 88, 256806 (2002)]. We show that this effect appears due to a specific magnetic control of the difference between the phase of the single nonresonant path via the free arm of the ring and the global phase of all trajectories involving resonant tunnelings through the dot.

64

Transport through a quantum ring, dot, and barrier embedded in a nanowire in magnetic field

Gudmundsson, V; Lin, YY; Tang, CS; Moldoveanu, V; Bardarson, JH; Manolescu, A

JUN 2005, PHYSICAL REVIEW B, 71

DOI: 10.1103/PhysRevB.71.235302

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We investigate the transport through a quantum ring, a dot, and a barrier embedded in a nanowire in a homogeneous perpendicular magnetic field. To be able to treat scattering potentials of finite extent in a magnetic field we use a mixed momentum-coordinate representation to obtain an integral equation for the multiband scattering matrix. For a large embedded quantum ring we are able to obtain Aharonov-Bohm type of oscillations with superimposed narrow resonances caused by interaction with quasibound states in the ring. We also employ the scattering matrix approach to calculate the conductance through a semiextended barrier or well in the wire. The numerical implementations we resort to in order to describe the cases of weak and intermediate magnetic field allow us to produce high resolution maps of the "near field" scattering wave functions, which are used to shed light on the underlying scattering processes.

65

Resonant and coherent transport through Aharonov-Bohm interferometers with coupled quantum dots

Moldoveanu, V; Tolea, M; Aldea, A; Tanatar, B

MAR 2005, PHYSICAL REVIEW B, 71

DOI: 10.1103/PhysRevB.71.125338

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A detailed description of the tunneling processes, within Aharonov-Bohm (AB) rings containing two-dimensional quantum dots is presented. We show that the electronic propagation through the interferometer is controlled by the spectral properties of the embedded dots and by their coupling with the ring. The transmittance of the interferometer is computed by the Landauer-Buttiker formula. Numerical results are presented for an AB interferometer containing two coupled dots. The charging diagrams for a double-dot interferometer and the Aharonov-Bohm oscillations are obtained, in agreement with the recent experimental results of Holleitner et al. [Phys. Rev. Lett. 87, 256802 (2001)] We identify conditions in which the system shows Fano line shapes. The direction of the asymetric tail depends on the capacitive coupling and on the magnetic field. We discuss our results in connection with the experiments of Kobayashi et al. [Phys. Rev. Lett. 88, 256806 (2002)] in the case of a single dot.

66

Tunneling properties of quantum dot arrays in a strong magnetic field

Moldoveanu, V; Aldea, A; Tanatar, B

AUG 2004, PHYSICAL REVIEW B, 70

DOI: 10.1103/PhysRevB.70.085303

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We study the transport properties of coherently coupled quantum dots in the quantum Hall regime within the Landauer-Buttiker formalism which captures and explains the experimentally observed features in terms of the spectral properties of the coupled dot system. The subpeak structure of the transmittance spectrum and the charging stability diagrams are obtained and discussed. The role of the intradot and interdot Coulomb interaction are pointed out. We show the subpeak evolution with the magnetic field and predict a specific oscillatory behavior of the Hall resistance in strong magnetic field which can be experimentally tested.

67

Orbital magnetization of single and double quantum dots in a tight-binding model

Aldea, A; Moldoveanu, V; Nita, M; Manolescu, A; Gudmundsson, V; Tanatar, B

JAN 15 2003, PHYSICAL REVIEW B, 67

DOI: 10.1103/PhysRevB.67.035324

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We calculate the orbital magnetization of single and double quantum dots coupled both by Coulomb interaction and by electron tunneling. The electronic states of the quantum dots are calculated in a tight-binding model, and the magnetization is discussed in relation to the energy spectrum and to the edge and bulk states. We identify effects of chirality of the electronic orbits and of the anticrossing of the energy levels when the magnetic field is varied. We also consider the effects of detuning the energy spectra of the quantum dots by an external gate potential. We compare our results with the recent experiments of Oosterkamp [Phys. Rev. Lett. 80, 4951 (1998)].

68

Dynamic correlation effects on the plasmon dispersion in a two-dimensional electron gas

Yurtsever, A; Moldoveanu, V; Tanatar, B

MAR 15 2003, PHYSICAL REVIEW B, 67

DOI: 10.1103/PhysRevB.67.115308

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The charge-density oscillations (plasmons) of a low-density two-dimensional uniform electron gas are studied within the framework of finite temperature and frequency dependent (dynamic) version of Singwi, Tosi, Land, and Sjolander theory and compared with the recent experimental results. The use of the Hartree-Fock approximation for the static structure factor leads to a finite temperature dynamical counterpart of the static Hubbard approximation. We observe important differences between dynamic and static local-field factors as well as between the corresponding plasmon dispersion laws. Our calculated plasmon energies that include dynamic correlations are in very good agreement with the recent experimental results.

69

Many-body effects in the Coulomb drag between low density electron layers

Yurtsever, A; Moldoveanu, V; Tanatar, B

MAR 2003, SOLID STATE COMMUNICATIONS, 125, 579

DOI: 10.1016/S0038-1098(03)00081-4

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Recent Coulomb drag experiments in low-density double-layer electron systems have the power of distinguishing various many-body formulations of the effective interactions. In this work we theoretically study the correlation effects on the drag resistivity in these systems within various models. The effective inter-layer interactions are best described by the generalization to the double-layer case of the Kukkonen-Overhauser approach which differs significantly from the self-consistent field approach of Singwi et al. [Phys. Rev. 176 (1968) 589]. Following the formulation of Vignale and Singwi [Phys. Rev. B 32 (1985) 2156] we derive an expression for the effective inter-layer interaction which embodies the many-body correlations through the local-field corrections. The drag resistivity is calculated within this approach together with the Hubbard approximation for the intra-layer local-field factor and a simple model for the inter-layer correlations. Comparison with the recent measurements of Kellogg et al. [Solid State Commun. 123 (2002) 5151 yields very good agreement. Our results are also contrasted with the corresponding drag resistivities given by the Singwi et al. theory, the dynamic random-phase approximation and the Hubbard approximation. The significant differences found between these theories emphasize the strong sensitivity of the drag resistivity to the effective inter-layer interactions. (C) 2003 Elsevier Science Ltd. All rights reserved.

70

Coulomb effects on the transport properties of quantum dots in a strong magnetic field

Moldoveanu, V; Aldea, A; Manolescu, A; Nita, M

JAN 15 2001, PHYSICAL REVIEW B, 63

DOI: 10.1103/PhysRevB.63.045301

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We investigate the transport properties of quantum dots placed in a strong magnetic field using a quantum-mechanical approach based on the two-dimensional tight-binding Hamiltonian with direct Coulomb interaction and the Landauer-Buttiker formalism. The electronic transmittance and the Hall resistance show Coulomb oscillations and also prove multiple addition processes. We identify this feature as the "bunching" of electrons observed in recent experiments and give an elementary explanation in terms of spectral characteristics of the dot. The spatial distribution of the added electrons may distinguish between the edge and bulk states and it has specific features for bunched electrons. The dependence of the charging energy on the number of electrons is discussed for a strong magnetic field. The crossover from the tunneling to quantum Hall regime is analyzed in terms of dot-lead coupling.